Efficiency of low-temperature adsorptive hydrogen storage systems (Englisch)

In: International Journal of Hydrogen Energy   ;  39 ,  28  ;  15604-15613  ;  2014
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  • Aufsatz (Zeitschrift)  /  Elektronische Ressource

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Abstract This study presents a thermodynamic analysis of adsorptive hydrogen storage systems at cryogenic temperatures, focusing mainly on the efficiency of the storage system. Four different operation modes, differing in the process used to release the hydrogen and the availability of cooling during storage time, are examined. A sensitivity analysis was performed to determine the dependency of the efficiency on several input parameters including storage time, enthalpy of adsorption, energy required for cooling, and system size. It can be concluded that the energetic efficiency of the hydrogen storage system not considering production and usage steps ranges from 65 to 81% for short storage times, depending on the energy effort and hydrogen losses of the applied operation mode. The storage time has the most noticeable impact on efficiency and cryo-adsorptive hydrogen storage is not suitable for long storage times due to the increasing cooling effort or hydrogen losses. For short storage times e.g. hours, cooling during storage time may be omitted due to the low hydrogen losses.

Highlights Efficiency of adsorptive hydrogen storage at cryogenic temperatures is determined. Efficiency is between 65 and 81% for short storage times. Efficiency drops with increasing storage time, long-term storage not meaningful. Efficiency of uncooled storage increases with system size and heat of adsorption.

Inhaltsverzeichnis – Band 39, Ausgabe 28

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Wang, Dan / Zhang, Xin-Tong / Sun, Pan-Pan / Lu, Shan / Wang, Ling-Ling / Wei, Yong-An / Liu, Yi-Chun | 2014
16220
Comparison between the measured and modeled hydrogen-evolution activity of Ni- or Pt-coated silicon photocathodes
Huang, Zhuangqun / McKone, James R. / Xiang, Chengxiang / Grimm, Ronald L. / Warren, Emily L. / Spurgeon, Joshua M. / Lewerenz, Hans-Joachim / Brunschwig, Bruce S. / Lewis, Nathan S. | 2013
16227
Interface functionalization with polymer self-assembly to boost photovoltage of Cu2O/ZnO nanowires solar cells
Xie, Jiale / Guo, Chunxian / Li, Chang Ming | 2014
16234
Clathrate hydrates for hydrogen storage: The impact of tetrahydrofuran, tetra-n-butylammonium bromide and cyclopentane as promoters on the macroscopic kinetics
Veluswamy, Hari Prakash / Chin, Weng Inn / Linga, Praveen | 2014
16244
Hydrogen storage in porous graphene with Al decoration
Ao, Zhimin / Dou, Shixue / Xu, Zhemi / Jiang, Quanguo / Wang, Guoxiu | 2014
16252
Anodic TiO2 nanotube array supported nickel – noble metal bimetallic catalysts for activation of CH4 and CO2 to syngas
Rui, Zebao / Feng, Danyan / Chen, Huayao / Ji, Hongbing | 2013
iii
Editorial Board
| 2014