Studies of oxide glass structure using laser ionization time of flight mass spectrometry (English)

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In: Journal of Physics: Condensed Matter   ;  15 ,  31  ;  S2323-S2334  ;  2003
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We report on our work on determining the structure of oxide glasses using laser ionization time of flight mass spectrometry. This technique is especially suitable for investigation of the intermediate-range order in glasses, where it can measure the presence and relative abundance of mesounits composed of 7–20 or more atoms. After introducing the experimental aspects and caveats of this new spectroscopy, we discuss the application of the instrument to a variety of heavy-metal oxide glass families. We separate our networks into those that have superstructural networks and those that show highly fragmented ones, including our studies of lead and bismuth borates, lead silicates, lead vanadates, and bismuth gallates. We also analyse our spectra for evidence of mixing in lead borosilicates, and to clarify the sharing of cations in sodium-doped lead borosilicates.

Table of contents – Volume 15, Issue 31

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Tables of content are generated automatically and are based on records of articles contained that are available in the TIB-Portal index. Due to missing records of articles, the volume display may be incomplete, even though the whole journal is available at TIB.

5341
Fluoride ion dynamics and relaxation in KSn2F5 studied by 19F nuclear magnetic resonance and impedance spectroscopy
M M Ahmad / M A Hefni / A H Moharram / G M Shurit / K Yamada / T Okuda | 2003
5353
The magnetoresistance of the quasi-one-dimensional conductor NbSe3
Jing-qin Shen / Xue-zhi Chen / Yi Zheng / Hong-tao Wang / Zhu-an Xu | 2003
5359
High-temperature thermoelectric performance of Si#8211Ge alloys
Tripathi, M.N. / Bhandari, C.M. | 2003
5359
High-temperature thermoelectric performance of Si–Ge alloys
M N Tripathi / C M Bhandari | 2003
5371
Onset of magnetism in Y1−xGdxCo2: effect on the heat capacity and electrical resistivity
N V Baranov / A A Yermakov / A Podlesnyak | 2003
5383
Role of different cap layers tuning the wavelength of self-assembled InAs/GaAs quantum dots
Z Gong / Z D Fang / X H Xu / Z H Miao / Z C Niu / S L Feng | 2003
5389
Electrical and thermal transport properties of (TlBiS2)1−x(2PbS)x alloys
N S Popovich / V K Shura | 2003
L483
Comparison of the Fermi-surface topologies of κ-(BEDT-TTF)2Cu(NCS)2 and its deuterated analogue
R S Edwards / A Narduzzo / J Singleton / A Ardavan / J A Schlueter | 2003
L491
Roles of local icosahedral chemical ordering in glass and quasicrystal formation in metallic glass formers
Hajime Tanaka | 2003
S2309
Dynamics of mobile ions in single- and mixed-cation glasses
C Cramer / S Brunklaus / Y Gao / K Funke | 2003
S2323
Studies of oxide glass structure using laser ionization time of flight mass spectrometry
Mario Affatigato / Steve Feller / Allison K Schue / Sarah Blair / Dale Stentz / Garret B Smith / Dan Liss / Matt J Kelley / Cole Goater / Raghuvir Leelesagar | 2003
S2335
The phonon density of states in amorphous materials
M Grimsditch / A Polian / R Vogelgesang | 2003
S2343
Thermochemistry of glasses along the 2NdAlO3–3SiO2 join
Yahong Zhang / Alexandra Navrotsky / Jean A Tangeman / J K Richard Weber | 2003
S2357
Local structure of Al-and Fe-based metallic glasses
Kyungsoo Ahn / Despina Louca / S J Poon / G J Shiflet | 2003
S2365
Biomolecular characterization of glass surfaces
Alexis G Clare / Matthew M Hall / Michelle L Korwin-Edson / Alan H Goldstein | 2003
S2377
Crack fronts and damage in glass at the nanometre scale
Christian Marlière / Silke Prades / Fabrice Célarié / Davy Dalmas / Daniel Bonamy / Claude Guillot / Elisabeth Bouchaud | 2003
S2387
Dependence of bridging oxygen 17O quadrupolar coupling parameters on Si–O distance and Si–O–Si angle
Ted M Clark / Philip J Grandinetti | 2003
S2397
Evidence for nanoscale phase separation of stressed–rigid glasses
S Mamedov / D G Georgiev / Tao Qu / P Boolchand | 2003
S2413
A neutron and x-ray diffraction study of calcium aluminate glasses
C J Benmore / J K R Weber / S Sampath / J Siewenie / J Urquidi / J A Tangeman | 2003
S2425
A quantitative measure of medium-range order in amorphous materials from transmission electron micrographs
R K Dash / P M Voyles / J M Gibson / M M J Treacy / P Keblinski | 2003
S2437
Approach to the glass transition studied by higher order correlation functions
N Lacević / S C Glotzer | 2003
S2447
Confocal fluorescence and Raman microscopy of femtosecond laser-modified fused silica
W Reichman / J W Chan / D M Krol | 2003
S2457
Site symmetry in binary and ternary tin silicate glasses—29Si and 119Sn nuclear magnetic resonance
D Holland / A P Howes / R Dupree / J A Johnson / C E Johnson | 2003
LETTER TO THE EDITOR: Roles of local icosahedral chemical ordering in glass and quasicrystal formation in metallic glass formers
Tanaka, Hajime | 2003
Preface
Johnson, Jacqueline A. | 2003
Evidence for nanoscale phase separation of stressed#8211rigid glasses
Mamedov, S. / Georgiev, D.G. / Qu, Tao / Boolchand, P. | 2003
LETTER TO THE EDITOR: Comparison of the Fermi-surface topologies of IMG entity="kappa" SRC="http: ej.iop.org-icons-Entities-kappa.gif" ALT="kappa" ALIGN="MIDDLE">-(BEDT-TTF)2Cu(NCS)2 and its deuterated analogue
Edwards, R.S. / Narduzzo, A. / Singleton, J. / Ardavan, A. / Schlueter, J.A. | 2003
Dependence of bridging oxygen 17O quadrupolar coupling parameters on Si#8211O distance and Si#8211O#8211Si angle
Clark, Ted M. / Grandinetti, Philip J. | 2003
Site symmetry in binary and ternary tin silicate glasses#821229Si and 119Sn nuclear magnetic resonance
Holland, D. / Howes, A.P. / Dupree, R. / Johnson, J.A. / Johnson, C.E. | 2003
Thermochemistry of glasses along the 2NdAlO3#82113SiO2 join
Zhang, Yahong / Navrotsky, Alexandra / Tangeman, Jean A. / Weber, J.K.Richard | 2003