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Inhaltsverzeichnis
6595
Titelbild: A Highly Emissive Fluorescent Nucleoside that Signals the Activity of Toxic Ribosome‐Inactivating Proteins (Angew. Chem. 35/2008)
Srivatsan, Seergazhi G.
/ Greco, Nicholas J.
/ Tor, Yitzhaket al.
| 2008
Innentitelbild: A Discrete Supramolecular Conglomerate Composed of Two Saddle‐Distorted Zinc(II)‐Phthalocyanine Complexes and a Doubly Protonated Porphyrin with Saddle Distortion Undergoing Efficient Photoinduced Electron Transfer (Angew. Chem. 35/2008)
Kälte- und druckinduzierte Dissoziation von Proteinaggregaten und Amyloidfibrillen Unsere Arbeiten werden von der Deutschen Forschungsgemeinschaft (DFG) und dem Fonds der Chemischen Industrie unterstützt.
Nickel-Mediated Coupling Reactions of Carboryne with Alkenes: A Synthetic Route to Alkenylcarboranes This work was supported by grants from the Research Grants Council of the Hong Kong Special Administration Region (Project No. 403805) and a Strategic Investments Scheme administrated by The Chinese University of Hong Kong.
High-Pressure Entry into Platencin This research has been financially supported (in part) by the Council for Chemical Sciences of The Netherlands Organization for Scientific Research (NWO-CW). We would like to thank J. M. M. Smits (Institute for Molecules and Materials, Radboud University Nijmegen) for the crystallographic analysis.
Total Syntheses and Structural Revision of α- and β-Diversonolic Esters and Total Syntheses of Diversonol and Blennolide C We thank Dr. R. K. Chadha, Dr. D. H. Huang, and Dr. G. Siuzdak for X-ray crystallographic, NMR spectroscopic, and mass spectrometric assistance, respectively. We also gratefully acknowledge Prof. S. Bräse and Prof. R. J. Capon for providing the spectra of synthetic diversonol and natural rugulotrosins, respectively, as well as Dr. D. J. Edmonds and Dr. A. F. Lenzen for helpful discussions. This work was supported by the National Institutes of Health, the Skaggs Institute for Chemical Biology, and a Bristol-Myers Squibb Graduate Fellowship (to A.L.).
Hydrocarbon Chain Growth on V(100) Single-Crystal Surfaces via Vinyl Intermediates Funding for this work was provided by the U.S. National Science Foundation.
Synthesis of Enantioenriched α-(Hydroxyalkyl)-tri-n-butylstannanes We thank the NIH (GM31278, DK38226) and the Robert A. Welch Foundation for financial support.
Efficient Fixation of Carbon Dioxide by Hypervalent Organobismuth Oxide, Hydroxide, and Alkoxide This work was supported in part by Japan Society for the Promotion of Science (JSPS) and Grant-in-Aid for Scientific Research on Priority Areas (No. 19027054, Synergy of Elements) from Ministry of Education, Culture, Sports, Science and Technology (Japan). S.F.Y. thanks JSPS for a postdoctoral fellowship. We thank Mr. Toshifumi Tanaka for his help. We are grateful to the reviewers for their valuable suggestions.
[1,5]-Hydride Transfer-Cyclizations on Alkynyl Fischer Carbene Complexes: Synthesis of 1,2-Dihydroquinolinyl Carbene Complexes and Cascade Reactions Financial support from the DGICYT (CTQ2007-61048-BQU). A FPU predoctoral fellowship to M.F.-M. is gratefully acknowledged. We also thank Dr. Angel L. Suárez for help in the X-ray structure determination.
Fast Reductive Ligation of S-Nitrosothiols We thank the Washington State University for supporting this work. We also thank Prof. P. Garner and Prof. R. Ronald for helpful discussions.
Parallel Synthesis and Screening of Polymer-Supported Phosphorus-Stereogenic Aminophosphane-Phosphite and -Phosphinite Ligands This work was supported by the NWO Combinatorial Chemistry program and DSM. J. M. Ernsting is acknowledged for assistance with NMR data analysis.
Syntheses, Structures, and Reactivities of Borylcopper and ‐zinc Compounds: 1,4‐Silaboration of an α,β‐Unsaturated Ketone to Form a γ‐Siloxyallylborane
Syntheses, Structures, and Reactivities of Borylcopper and -zinc Compounds: 1,4-Silaboration of an α,β-Unsaturated Ketone to Form a γ-Siloxyallylborane This work was supported by a Grant-in-Aid for Scientific Research on Priority Areas (No. 17065005, "Advanced Molecular Transformations of Carbon Resources" and No. 19027015, "Synergy of Elements") and for Young Scientists (B) (18750027) from MEXT (Japan) and by Kurata Memorial Hitachi Science and Technology Foundation. T.K. thanks AGC Corporation for financial support.
Syntheses, Structures, and Reactivities of Borylcopper and -zinc Compounds: 1,4-Silaboration of an a,b-Unsaturated Ketone to Form a g-Siloxyallylborane
Kajiwara, T.
/ Terabayashi, T.
/ Yamashita, M.et al.
| 2008
Quasi-Elastic Neutron Scattering and Molecular Dynamics Study of Methane Diffusion in Metal Organic Frameworks MIL-47(V) and MIL-53(Cr) This work was supported by the French program ANR CO2 "NoMAC" (ANR-06-CO2-008) and European funding ALFA II "NANOGASTOR" (II-0493-FA-FI). We thank the Institut Laue-Langevin (Grenoble, France) for the neutron beam time, Dr. M. M. Koza for his help, and the CINES for computational facility.
Toward Fluorescent Memories with Nondestructive Readout: Photoswitching of Fluorescence by Intramolecular Electron Transfer in a Diaryl Ethene‐Perylene Bisimide Photochromic System
Toward Fluorescent Memories with Nondestructive Readout: Photoswitching of Fluorescence by Intramolecular Electron Transfer in a Diaryl Ethene-Perylene Bisimide Photochromic System Financial support from MUR (PRIN 2006 030320) is gratefully acknowledged. We thank S. Carli for preliminary synthetic work and C. Chiorboli for help with the femtosecond studies.
Germanium(II)-Mediated Reductive Mannich-Type Reaction of α-Bromoketones to N-Alkylimines This work was supported by a Grant-in-Aid for Scientific Research from the Ministry of Education, Culture, Sports, Science and Technology of the Japanese Government. S.T. expresses his special thanks for Research Fellowships of the Japan Society for JSPS Research Fellowships for Young Scientists.
Evidence for an Enol Mechanism in a Highly Enantioselective Mannich-Type Reaction Catalyzed by Primary Amine-Thiourea We gratefully acknowledge generous financial support from the Deutsche Forschungsgemeinschaft (SPP 1179 "Organocatalysis") and generous amount of computational time from HLRBII (LRZ).
CdS Nanoparticles-β-Cyclodextrin-Functionalized Electrodes for Enhanced Photoelectrochemistry This study was supported by the NanoSci-ERA program, administered by the EC and the Israel Science Foundation.
Asymmetric Diels-Alder Reactions of α,β-Unsaturated Aldehydes Catalyzed by a Diarylprolinol Silyl Ether Salt in the Presence of Water This work was partially supported by the Toray Science Foundation, and a Grant-in-Aid for Scientific Research from MEXT. S.S. is grateful to the Japan Society for the Promotion of Science (JSPS) for a postdoctoral fellowship.
Ruthenium Porphyrin-Catalyzed Aerobic Oxidation of Terminal Aryl Alkenes to Aldehydes by a Tandem Epoxidation-Isomerization Pathway We are thankful for the financial support of The University of Hong Kong (University Development Fund), the University Grants Council of HKSAR (the Area of Excellence Scheme: AoE 10-01P), the Hong Kong Research Grants Council (HKU7009-06P and CityU 2-06C), and CAS-Croucher Funding Scheme for Joint Laboratory. G.J. and J.C. thank the Croucher Foundation of Hong Kong for a postgraduate studentship.
[Ru(phgly)2(binap)]-Li2CO3: A Highly Active, Robust, and Enantioselective Catalyst for the Cyanosilylation of Aldehydes This work was supported by Grants-in-Aid from the Japan Society for the Promotion of Science (JSPS) (No. 18350046) and the Innovation Plaza Hokkaido in the Japan Science and Technology Agency (JST). phgly=phenylglycinate, binap=2,2'-bis(diphenylphosphanyl)-1,1'-binapht- hyl.
Catalytic Enantioselective Trapping of an Alcoholic Oxonium Ylide with Aldehydes: RhII/ZrIV‐Co‐Catalyzed Three‐Component Reactions of Aryl Diazoacetates, Benzyl Alcohol, and Aldehydes
Catalytic Enantioselective Trapping of an Alcoholic Oxonium Ylide with Aldehydes: RhII-ZrIV-Co-Catalyzed Three-Component Reactions of Aryl Diazoacetates, Benzyl Alcohol, and Aldehydes We are grateful for financial support from the National Science Foundation of China (Grant No. 20772033) and for sponsorship by the Shanghai Pujiang Program.
Rapid Construction of the Cortistatin Pentacyclic Core We are grateful to UC Berkeley and GlaxoSmithKline for supporting this research. E.M.S. acknowledges the ACS Division of Medicinal Chemistry and Eli Lilly for a predoctoral fellowship.
Patterns of Electrostatic Charge and Discharge in Contact Electrification This research was supported by the Department of Energy, Division of Materials Science and Engineering under award DE-FG02-00 ER45852, and by the Army Research Office with a MURI (W911NF-04-1-0170). We also acknowledge the Xerox Corporation for financial support, Prof. Zhigang Suo and Xuanhe Zhao for helpful discussions, as well as the American Cancer Society (S.W.T.) and NSERC of Canada (S.J.V.) for postdoctoral fellowships.
The Asymmetric Total Synthesis of (+)-Cytotrienin A, an Ansamycin-Type Anticancer Drug This work was supported by a Grant-in-Aid for Creative Scientific Research from The Ministry of Education, Culture, Sports, Science, and Technology (MEXT).
A Highly Emissive Fluorescent Nucleoside that Signals the Activity of Toxic Ribosome-Inactivating Proteins We are grateful to the National Institutes of Health (grant number GM069773) for support.
An Organometallic Approach to Gold Nanoparticles: Synthesis and X-Ray Structure of CO-Protected Au21Fe10, Au22Fe12, Au28Fe14, and Au34Fe14 Clusters Financial support from the University of Bologna (Clustercat), the MIUR (PRIN2006), and PRRIITT (Nanofaber) is gratefully acknowledged. We wish to thank Dr. Magda Blosi for her support with the DLS measurements.
Solving Complex Concentric Circular Mesostructures by Using Electron Tomography We thank the State Key Research Program (2004CB217804, 2006CB932302), the NSFC (20721063, 20573021), SLADP (B108), NCET, and the Australian Research Council for financial support. We thank Dr. Matthias Floetenmeyer (UQ) for help with the ultramicrotome experiments.
Solid-Phase Organic Synthesis in the Presence of Compressed Carbon Dioxide Financial support from the Fonds der Chemischen Industrie and the Max-Buchner-Foundation (A.S.) is gratefully acknowledged.
Helical Peptide Arrays on Self-Assembled Monolayer Surfaces through Soft and Reactive Landing of Mass-Selected Ions This work was supported by the Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory and a grant from the Chemical Sciences Division, Office of Basic Energy Sciences of the U.S. Department of Energy. The authors thank Dr. John Cort for technical assistance and helpful discussions.
Nanohybrid Carbon Film for Electrochemical Detection of SNPs without Hybridization or Labeling This work was supported by the CREST-JST project. SNP=single-nucleotide polymorphism.
Dissociation of SO2 on Au-TiC(001): Effects of Au-C Interactions and Charge Polarization The research carried out at BNL was supported by the US Department of Energy, Chemical Sciences Division. J.A.R. acknowledges the support of the Generalitat de Catalunya in a visit to the Universitat de Barcelona. F.V. thanks the Spanish Ministry of Education and Science and Universitat de Barcelona for supporting his predoctoral research. K.N. thanks the Nippon Foundation for Materials Science for grants that made possible part of this work. Computational time on the Marenostrum supercomputer of the Barcelona Supercomputing Center is gratefully acknowledged.
Peristaltic Motion of Polymer Gels This work was supported in part by "The innovative research on symbiosis technologies for human and robots in the elderly dominated society," 21st Century Center of Excellence (COE) Program Japan Society or the Promotion of Science; "Establishment of Consolidated Research Institute for Advanced Science, and Medical Care", Encouraging Development Strategic Research Centers Program, the Special Coordination Funds for Promoting Science and Technology, Ministry of Education, Culture, Sports, Science, and Technology (Japan) and "Fundamental Study for Intelligent Machines to Coexist with Nature", Advanced Research Institute for Science and Engineering, Waseda University.
Covalently Linked Dimers of Clusters: Loop- and Dumbbell-Shaped Mn24 and Mn26 Single-Molecule Magnets This work was supported by the U.S. National Science Foundation (Grant CHE-0414555).
Observation of Electrochemical Single-Electron-Transfer Events of Gold Nanoparticles in Aqueous Solution in the Presence of Both Ammonium and Sulfonate Surface-Active Agents The authors thank Mr. T. Takasaki and Ms. E. Kagami (Rigaku) for the SAXS measurements and Mr. F. Toshimitsu (Univ. Tokyo) for STM analysis. This work was supported by Japan Science and Technology (JST) Agency and Hayashi Memorial Foundation for Female Nature Scientists.
Observation of Electrochemical Single‐Electron‐Transfer Events of Gold Nanoparticles in Aqueous Solution in the Presence of Both Ammonium and Sulfonate Surface‐Active Agents
Functional Analysis of an Aspartate-Based Epoxidation Catalyst with Amide-to-Alkene Peptidomimetic Catalyst Analogues We thank the NIH (National Institute of General Medical Sciences) and Merck Research Laboratories, each for partial support.
A Discrete Supramolecular Conglomerate Composed of Two Saddle‐Distorted Zinc(II)‐Phthalocyanine Complexes and a Doubly Protonated Porphyrin with Saddle Distortion Undergoing Efficient Photoinduced Electron Transfer
A Discrete Supramolecular Conglomerate Composed of Two Saddle-Distorted Zinc(II)-Phthalocyanine Complexes and a Doubly Protonated Porphyrin with Saddle Distortion Undergoing Efficient Photoinduced Electron Transfer The support of Grants-in-Aid (Nos. 18033033, 19205019, 19655045, and 19750034) from the Ministry of Education, Culture, Sports, Science and Technology (Japan) is gratefully acknowledged. We also appreciate a support from Japan Science and Technology Agency (JST) through the "potentiality verification stage" program.
Site-Selective Fabrication of Two-Dimensional Fullerene Arrays by Using a Supramolecular Template at the Liquid-Solid Interface Financial support from the National Natural Science Foundation of China (grant nos. 90406019, 20473097, and 20573116) and the National Key Project for Basic Research (grant nos. 2007CB936503 and 2007CB936802) is gratefully acknowledged.