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The purpose of the study was to identify potential water quality problems associated with runoff and percolation through mine spoils at selected sites in the Upper Colorado River Basin. The results show that the production of soluble salts from mine spoils into receiving waters is probably the most significant water quality problem that can be expected. No significant release of heavy metals was observed in the coal mine spoils studied. Some significant heavy metal concentrations were observed in the stream below the tailings disposal area from a copper-lead-zinc mill. A portion of these metals are contributed by the tailings, but a variety of old mines and mine dumps also make a contribution. The quality of percolate and runoff from spoils was found to correspond to the constituents of extracts prepared from saturated pastes of the spoil material. A method of estimating salt production into receiving waters was derived and found to agree very well with measured salt pickup at one coal site. The minimum quantities of salts that will eventually be released from the spoils studied are estimated.