Femtosecond laser electronic excitation tagging (FLEET) velocimetry and laser Rayleigh scattering are conducted concurrently and are evaluated for their suitability to measure velocity and density simultaneously in NASA Langley’s 0.3-m Transonic Cryogenic Tunnel. FLEET velocimetry measurements are shown to be accurate to within 1.5 percent of the measured velocity throughout the facility testing envelope and exhibit a zero-velocity precision of 0.4 m/s. Rayleigh scattering density measurements indicate a characteristically linear dependence on flow density while having an accuracy within 5.4 percent of the measured density and a precision less than or equal to 6 percent. The preliminary assessment indicates that the joint technique would be advantageous for deployment in high-pressure, cryogenic test facilities.