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3707
Titelbild: Zipper Assembly of Vectorial Rigid-Rod p-Stack Architectures with Red and Blue Naphthalenediimides: Toward Supramolecular Cascade n/p-Heterojunctions (Angew. Chem. 20/2008)
Sisson, A. L.
/ Sakai, N.
/ Banerji, N.et al.
| 2008
Titelbild: Zipper Assembly of Vectorial Rigid‐Rod π‐Stack Architectures with Red and Blue Naphthalenediimides: Toward Supramolecular Cascade n/p‐Heterojunctions (Angew. Chem. 20/2008)
Sisson, Adam L.
/ Sakai, Naomi
/ Banerji, Natalieet al.
| 2008
Ferrocenylliganden mit zwei Phosphanylsubstituenten in α,ε‐Position für die Übergangsmetall‐katalysierte asymmetrische Hydrierung funktionalisierter Doppelbindungen
Ferrocenylliganden mit zwei Phosphanylsubstituenten in a,?-Position fur die Ubergangsmetall-katalysierte asymmetrische Hydrierung funktionalisierter Doppelbindungen
Ireland, T.
/ Grossheimann, G.
/ Wieser-Jeunesse, C.et al.
| 2008
Reply to "Mirror Symmetry Breaking" of the Centrosymmetric CaCO3 Crystals with Amino AcidsFNR HREF="nss"> FN ID="nss"> This research was supported by the Deutsche Forschungs-gemeinschaft (DFG) within the priority program "Principles of Biomineralization". S. E. Wolf is recipient of a Konrad Adenauer fellowship. We are grateful to Prof. Dr. W. Hofmeister for access to the SEM facilities.
A Bioluminescent Molecular Switch For GlucoseFNR HREF="nss"> FN ID="nss"> This work was supported in part by grants from the National Institutes of Health and the National Aeronautics and Space Administration. We thank the Office of the Vice President of Research at the University of Kentucky for a University Research Professorship to S.D. K.T. acknowledges support from a Gill Fellowship, and S.D. from a Gill Eminent Professorship.
Simultaneous Determination of the Conformation and Relative Configuration of Archazolide A by Using Nuclear Overhauser Effects, J Couplings, and Residual Dipolar Couplings
Simultaneous Determination of the Conformation and Relative Configuration of Archazolide A by Using Nuclear Overhauser Effects, J Couplings, and Residual Dipolar CouplingsFNR HREF="nss"> FN ID="nss"> This work was supported by the Max-Planck-Gesellschaft, the Volkswagenstiftung (Funding Initiative: "Interplay between Molecular Conformations and Biological Function"), and the Fonds der Chemischen Industrie ("Liebig-Stipendium" to D.M.). We thank Tatjana Arnold for technical support and Dr. Peter Harberz for his precious help in the preparation of the PH gel.
Zipper Assembly of Vectorial Rigid-Rod π-Stack Architectures with Red and Blue Naphthalenediimides: Toward Supramolecular Cascade n-p-HeterojunctionsFNR HREF="nss"> FN ID="nss"> We thank S. Bhosale and D.-H. Tran for contributions to synthesis, D. Jeannerat, A. Pinto and S. Grass for NMR measurements, P. Perrottet and the group of F. Gülaçar, N. Oudry, and G. Hopfgartner for MS, one referee for helpful comments, and the Swiss NSF for financial support.
Water-Soluble Nanocrystals Through Dual-Interaction LigandsFNR HREF="nss"> FN ID="nss"> We thank Prof. Randolph Duran and Dr. Jorge Chávez for DLS measurements, and Dr. Yunjun Wang for helpful discussions. Y.C.C. acknowledges the NSF (DMR-0645520 Career Award), ONR (N00014-06-1-0911) and the American Chemical Society Petroleum Research Fund (42542-G10) for support of this research.
A Highly Selective Luminescent Switch-On Probe for Histidine-Histidine-Rich Proteins and Its Application in Protein StainingFNR HREF="nss"> FN ID="nss"> This research was supported by The Hong Kong Polytechnic University and the Area of Excellence Fund of the University Grants Committee (AoE-P-10-01). D.L.M. and W.L.W. acknowledge the award of postdoctoral fellowships administered by the Research Committee of The Hong Kong Polytechnic University. We are grateful to Prof. Chi-Ming Che for supporting this research and for his invaluable suggestions.
1,2,3-Triazole CH···Cl- Contacts Guide Anion Binding and Concomitant Folding in 1,4-Diaryl Triazole OligomersFNR HREF="nss"> FN ID="nss"> This work was supported by Duke University. We thank T. Ribeiro for assistance with 2D NMR experiments.
A Caged Retinoic Acid for One- and Two-Photon Excitation in Zebrafish EmbryosFNR HREF="nss"> FN ID="nss"> We thank B. Lesaffre and F. Rosa for access to their fish data and facility. This work was supported by the Association pour la Recherche sur le Cancer (ARC, contract no. 3787). The authors declare no competing financial interests.
Development of Selective RabGGTase Inhibitors and Crystal Structure of a RabGGTase-Inhibitor ComplexFNR HREF="nss"> FN ID="nss"> RabGGTase: Rab geranylgeranyl transferase. We thank the X-ray communities of the Max-Planck-Institut für molekulare Physiologie (Dortmund, Germany) and the Max-Planck-Institut für medizinische Forschung (Heidelberg, Germany) for collecting diffraction data at the Swiss Light Source of the Paul Scherrer Institute (Villigen, Switzerland) and for giving us generous access and support for the station X10SA. K.A. was supported by a Heisenberg Award of the Deutsche Forschungsgemeinschaft (DFG). This work was supported in part by DFG grants to K.A. (grant no.: AL 484-7-2) and to K.A., R.S.G, and H.W. (grant no.: SFB642), and by the Zentrum für Angewandte Chemische Genomik. R.S.B. thanks the Alexander von Humboldt Stiftung for a scholarship.
Protein-Cross-Linked Polymeric Materials through Site-Selective BioconjugationFNR HREF="nss"> FN ID="nss"> We gratefully acknowledge the Biomolecular Materials Program at LBNL and the UCB Chemical Biology Graduate Program for generous financial support. We also thank Prof. Jean M. Fréchet and Prof. Carolyn R. Bertozzi for the use of instrumentation and equipment.
Synthesis of (-)-Octalactin A by a Strategic Vanadium-Catalyzed Oxidative Kinetic ResolutionFNR HREF="nss"> FN ID="nss"> We gratefully acknowledge the University of California, Berkeley, NIHGMS (grant no. R01 GM074774), Merck Research Laboratories, Bristol-Myers Squibb, Amgen Inc., and Novartis for financial support. We thank Prof. E. Vedejs and Dr. S. T. Staben for helpful discussions.
A Concise Synthesis of (-)-OseltamivirFNR HREF="nss"> FN ID="nss"> We thank the National Institutes of Health (GM 033049) and the National Science Foundation for their generous support of our programs. T.Z. thanks Novartis for a graduate fellowship. Mass spectra were provided, in part, by the Mass Spectrometry Regional Center of the University of California, San Francisco. Palladium salts were generously supplied by Johnson-Matthey. We are indebted to Dr. Kiran Guthikonda, David N. Zalatan, and Prof. Justin Du Bois for valuable discussions and donation of chemicals for the aziridination step. We thank Gilead Sciences for a reference sample of Tamiflu.
Total Synthesis of (+)-Oocydin A: Application of the Suzuki-Miyaura Cross-Coupling of 1,1-Dichloro-1-alkenes with 9-Alkyl 9-BBNFNR HREF="nss"> FN ID="nss"> Financial support from the Institut de Chimie des Substances Naturelles, CNRS is acknowledged. 9-BBN=9-borabicyclo[3.3.1]nonane.
Heterobimetallic Cooperation Mediates the Transformation of White Phosphorus into Zwitterionic catena-Phosphonium(+)diphosphenide(-) LigandsFNR HREF="nss"> FN ID="nss"> We are grateful to Thermphos International BV, Vlissingen (Netherlands), for a generous loan of white phosphorus. Our thanks also go to the NMR service of "Firenze Hydrolab", a project sponsored by Ente Cassa di Risparmio di Firenze. Dr. Andrea Raffaelli (ICCOM CNR, Pisa, Italy) is acknowledged for running the ESI-MS experiments.
A Transient VIII-Alkylidene Complex: Oxidation Chemistry Including the Activation of N2 to Afford a Highly Porous Honeycomb-Like FrameworkFNR HREF="nss"> FN ID="nss"> We thank Indiana University-Bloomington, the Dreyfus Foundation, the Sloan Foundation, and the US NSF for financial support of this research. U.J.K. acknowledges Baxter Pharmaceutical Co. for financial support, and Dr. John Tomaszewski for aid in NMR spectroscopic measurements. Prof. Amar Flood and Edward Witlicki are thanked for help with Raman spectra.
The "Complex-in-a-Complex" Cations [(acac)2M⊂Ru6(p-iPrC6H4Me)6(tpt)2(dhbq)3]6+: A Trojan Horse for Cancer CellsFNR HREF="nss"> FN ID="nss"> This work was supported by the Fonds National Suisse de la Recherche Scientifique. A generous loan of ruthenium trichloride hydrate from Johnson Matthey Technology Centre is gratefully acknowledged. M=Pd, Pt; acac=acetylacetonato; tpt=2,4,6-tris(pyridin-4-yl)-1,3,5-triazine; dhbq=2,5-dihydroxy-1,4-benzoquinonato.
Enantioselective Copper-Catalyzed Propargylic AminationFNR HREF="nss"> FN ID="nss"> The National Research School Combination-Catalysis (NRSC-C) is gratefully acknowledged for financial support of this project.
Copper-Catalyzed Asymmetric Propargylic Substitution Reactions of Propargylic Acetates with AminesFNR HREF="nss"> FN ID="nss"> This work was supported by Grant-in-Aids for Scientific Research for Young Scientists (S) (No. 19675002) and for Scientific Research on Priority Areas (No. 18066003) from the Ministry of Education, Culture, Sports, Science and Technology (Japan). G.H. acknowledges the Global COE Program for Chemistry Innovation. Y.N. also thanks to the Iketani Science & Technology Foundation and the Japan Securities Scholarship Foundation. We thank Mr. Yusuke Shimada for some experiments at the initial stage of this work.
An Annulation Reaction for the Synthesis of Morpholines, Thiomorpholines, and Piperazines from β-Heteroatom Amino Compounds and Vinyl Sulfonium SaltsFNR HREF="nss"> FN ID="nss"> M.Y. thanks the Higher Education Commission of Pakistan for support of a studentship. V.K.A. thanks the Royal Society for a Wolfson Research Merit Award and the EPSRC for a Senior Research Fellowship.
A Chiral Hypervalent Iodine(III) Reagent for Enantioselective Dearomatization of PhenolsFNR HREF="nss"> FN ID="nss"> This work was partially supported by a Grant-in-Aid for Scientific Research (A) and for Encouragement of Young Scientists, and by Scientific Research on Priority Areas "Advanced Molecular Transformations of Carbon Resources" from the Ministry of Education Culture, Sports, Science, and Technology (Japan). T.D. and A.M. acknowledge support from the Industrial Technology Research Grant Program from the New Energy and Industrial Technology Development Organization (NEDO) of Japan and a research fellowship from J.S.P.S. for Young Scientists.
The Versatile Chemistry and Noncentrosymmetric Crystal Structures of Salt-Inclusion Vanadate HybridsFNR HREF="nss"> FN ID="nss"> This work was supported by the National Science Foundation (NSF) (grant nos. DMR-0322905 and 0706426). Support from the NSF for the Summer Research Program in Solid State and Materials Chemistry (for R.P.; grant no. DMR-0303450), as well as the purchase of a SQUID magnetometer and an X-ray diffractometer, are also gratefully acknowledged. The authors are indebted to Prof. P. Shiv Halasyamani and Jaewook Baek of the University of Houston for their assistance in SHG measurements and to P.S.H. for invaluable discussions.
Enantioselective O-Nitroso Aldol Reaction of Silyl Enol EthersFNR HREF="nss"> FN ID="nss"> Support of this research was provided by National Institutes of Health (NIH) (Grant No. GM068433-01) and Merck Research Laboratories. M.K. thanks the Uehara Memorial Foundation for financial support.
The Influence of Guanine on DNA Hole Transport EfficiencyFNR HREF="nss"> FN ID="nss"> This research was supported by the Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, DOE under grants No. DE-FG02-96ER14604 (F.D.L.) and DE-FG02-99ER14999 (M.R.W.).
The Low Basicity of Phosphabenzenes: First Examples of Protonation, Alkylation, and Silylation ReactionsFNR HREF="nss"> FN ID="nss"> This work was supported by the National Science Foundation (C.A.R.) and the EPSRC (J.F.N., J.C.G.) and the Oxford Supercomputer Centre. We thank Dr. C. Tate, Dr. S. B Clendenning and Prof. F. G. N. Cloke for assistance with obtaining the tri- and monophosphabenzenes.
A Highly Efficient and Selective AuI-Catalyzed Tandem Synthesis of Diversely Substituted Pyrrolo[1,2-a]quinolines in Aqueous MediaFNR HREF="nss"> FN ID="nss"> This study was supported by The University of Hong Kong (University Development Fund), the Hong Kong Research Grants Council, and the University Grants Committee of the Hong Kong SAR of China (Area of Excellence Scheme, AoE-P-10-01)
Fluorescence-Quenching-Based Enzyme-Activity Assay by Using Photon UpconversionFNR HREF="nss"> FN ID="nss"> This study was supported by the Academy of Finland (grant nos.: 114903 and 119497). The authors thank Pirjo Laaksonen (University of Turku) for blood sampling and Hidex Oy for technological support in the anti-Stokes photoluminescence measurements.
Large-Scale Synthesis of Ultrathin Bi2S3 Necklace NanowiresFNR HREF="nss"> FN ID="nss"> G.A.O. is Canada Research Chair in Materials Chemistry. The authors are deeply indebted to the NSERC for financial support. L.C. thanks the University of Toronto for a scholarship. R.M. thanks the Iranian Ministry of Science, Research and Technology for a scholarship and F. Farzaneh for support
Katalytische asymmetrische C-Si-Bindungsknupfung an acyclischen a,b-ungesattigten Akzeptoren durch RhI-katalysierten konjugierten Silyltransfer mithilfe einer Si-B-Bindung
Katalytische asymmetrische C-Si-Bindungsknüpfung an acyclischen α,β-ungesättigten Akzeptoren durch RhI-katalysierten konjugierten Silyltransfer mithilfe einer Si-B-BindungFNR HREF="nss"> FN ID="nss"> Wir danken der Deutschen Forschungsgemeinschaft (Oe 249-3-1) für finanzielle Unterstützung sowie der Solvias AG (Basel) und der Saltigo GmbH (Leverkusen) für die Überlassung zahlreicher Liganden. Barbara Hildmann, Kristine Müther und Patrick Seelheim leisteten geschickte experimentelle Unterstützung. M.O. dankt der Aventis Foundation für ein Karl-Winnacker-Stipendium (2006-2008).
Katalytische asymmetrische C‐Si‐Bindungsknüpfung an acyclischen α,β‐ungesättigten Akzeptoren durch RhI‐katalysierten konjugierten Silyltransfer mithilfe einer Si‐B‐Bindung
Walter, Christian
/ Oestreich, Martinet al.
| 2008
Ein hierarchisch selbstorganisiertes Wirt-Gast-Netzwerk an der Fest-flüssig-Grenzfläche für die Manipulation einzelner MoleküleFNR HREF="nss"> FN ID="nss"> Die Autoren danken der Deutschen Forschungsgemeinschaft für die finanzielle Unterstützung im Rahmen des SFB 569 und H. Hoster für die Analyse der Nahordnung.
Synthese eines paramagnetischen Polymers durch ringöffnende Polymerisation eines gespannten [1]VanadoarenophansFNR HREF="nss"> FN ID="nss"> Diese Arbeit wurde von der DFG gefördert. T.K. dankt dem FCI für ein Promotionsstipendium.
Fern-IR-spektroskopische Charakterisierung der Wechselwirkung zwischen Kationen und Anionen in ionischen FlüssigkeitenFNR HREF="nss"> FN ID="nss"> Diese Arbeit wurde unterstützt durch das Land Mecklenburg-Vorpommern und den Pakt für Forschung und Innovation des Bundesministeriums für Bildung und Forschung-Leibniz Forschungsgemeinschaft.