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Titelbild: Immunitat im Reagenzglas: Die Zauberkugel wird Wirklichkeit (Angew. Chem. 48/2006)
Preparation, Adsorption Properties, and Catalytic Activity of 3D Porous Metal–Organic Frameworks Composed of Cubic Building Blocks and Alkali‐Metal Ions
Starre anellierte Kohlenstoff-Schwefel-StrukturenFNR HREF="nss"> FN ID="nss"> Die Arbeiten wurden von der Dirección General de Investigación Spanien (CTQ2006-15456-C04-04-BQU) gefördert.
Enamine-Based Aldol Organocatalysis in Water: Are They Really "All Wet"?FNR HREF="nss"> FN ID="nss"> Comments to several reports on enamine-based organocatalysis of aldol reactions in water (Refs. BIBR HREF="bib6">6-BIBR HREF="bib12">12). We thank Prof. Dale L. Boger for helpful discussions during the preparation of this manuscript.
In Water or in the Presence of Water?FNR HREF="nss"> FN ID="nss"> Response to Correspondence by Janda and co-workers (see preceding article). The author thanks the referee for helpful suggestions. The work carried out on this subject was partially supported by the Toray Science Foundation and a Grant-in-Aid for Scientific Research on Priority Areas 16073219 from MEXT.
Synthesis of Platinum Nanocages by Using Liposomes Containing Photocatalyst MoleculesFNR HREF="nss"> FN ID="nss"> Sandia is multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DEAC04-94AL85000.
Microscopy-Based Mass Measurement of a Single Whole Virus in a Cylindrical Ion TrapFNR HREF="nss"> FN ID="nss"> This work was supported by grants from Academia Sinica and the National Science Council (grant no. NSC 93-3112-B-001-012-Y) of Taiwan, R.O.C. We thank C.-S. Chung for preparation of the vaccinia virus and F. P. Cui for technical assistance.
Lanthanitin: A Chiral Nanoball Encapsulating 18 Lanthanum Ions by Ferritin-Like AssemblyFNR HREF="nss"> FN ID="nss"> N.J. thanks KOSEF (grant No. R02-2002-000-00128-0 of the Basic Research Program), CMDS and Korea University for their financial support. K.S.J., Y.S.K, and Y.J.K are grateful to BK21 program. J.K. thanks the Korea Research Foundation for the grant (KRF 2003-070-C00029).
Reversible Control of Carbon Nanotube Aggregation for a Glucose Affinity SensorFNR HREF="nss"> FN ID="nss"> This work was supported by the National Science Foundation (grant CTS-0330350). The authors would like to thank E. Mock for help with DLS measurements.
Fluoroproline Flip-Flop: Regiochemical Reversal of a Stereoelectronic Effect on Peptide and Protein StructuresFNR HREF="nss"> FN ID="nss"> We acknowledge the financial support of the Herman Frasch Foundation (418-97HF), the NIH (5R01L071136-04), and the NSF (EEC-9731643). The CD spectropolarimeter, differential scanning calorimeter, and X-ray diffractometer were obtained with the assistance of NSF and NIH grants.
Imprinted Photonic Polymers for Chiral RecognitionFNR HREF="nss"> FN ID="nss"> The work was supported by the National Science Foundation of China (20473044, 20533050).
An Aptamer-Doxorubicin Physical Conjugate as a Novel Targeted Drug-Delivery PlatformFNR HREF="nss"> FN ID="nss"> This work was supported by Korea Science and Technology Foundation grant R01-2006-000-10818-0 (S.J. and V.B.) and USA National Institutes of Health grants CA 119349 (R.L., O.F., and V.B.) and EB 003647 (O.F.). We also thank Prof. C. S. Park for helpful discussions. This work is dedicated to the families of patients with cancer.
Diversity in Guanine-Selective DNA Binding Modes for an Organometallic Ruthenium Arene ComplexFNR HREF="nss"> FN ID="nss"> We thank the Wellcome Trust (Travelling Fellowship for H.L. and facilities in the Edinburgh Protein Interaction Centre), the University of Western Australia (Study Leave Grant for S.J.B.-P.), ORS (studentship for J.X.), RC-UK (Rasor), and Oncosense Ltd for support, and colleagues in EC COST Action D20 for stimulating discussions.
Time-Controlled Microfluidic Seeding in nL-Volume Droplets To Separate Nucleation and Growth Stages of Protein CrystallizationFNR HREF="nss"> FN ID="nss"> This work was supported by NIH Protein Structure Initiative Specialized Centers Grant GM074961 (ATCG3D) and the NIH (R01 EB001903). Use of the Advanced Photon Source was supported by the US Department of Energy (contract no. W-31-109-Eng-38). Use of the BioCARS Sector 14 was supported by the NIH National Center for Research Resources (grant number RR07707). GM-CA-CAT has been funded in whole or in part by the National Cancer Institute (Y1-CO-1020) and the National Institute of General Medical Sciences (Y1-GM-1104). Funding for functional and structural proteomics of SARS CoV-related proteins is provided through NIH-NIAID contract HHSN266200400058C. We thank Ruslan Sanishvili (GM-CA Cat station 23ID-D staff support) for technical assistance; Scott Lovell and Lance Stewart (deCODE Biostructures) for helpful assistance and discussions; Shu Moy (Midwest Center for Structural Genomics) for cloning work on Oligoendopeptidase F; Vanitha Subramanian (The Scripps Research Institute) for cloning, expression,
Dual-Mode Nanoparticle Probes for High-Performance Magnetic Resonance and Fluorescence Imaging of NeuroblastomaFNR HREF="nss"> FN ID="nss"> We thank Dr. H. S. Kwon and J.-M. Oh for TEM analyses (KBSI-Chuncheon), and Prof. J.-S. Suh, Prof. Y.-M. Huh (Yonsei), Dr. O. H. Han, and S. H. Kim for MRI (KBSI-Daegu). This work was supported in part by the National Research Laboratory (M10600000255), R&D Program for Cancer Control of Ministry of Health & Welfare (0320250-2), NCRC (R15-2004-024-00000-0), NCI Center for Nanotechnology Excellence, IT Leading R&D Support Project, AOARD-AFOSR, 2nd stage BK21 for Medical Science and Chemistry, and Korea Health 21 R&D Project of Ministry of Health & Welfare (A050260).
Design, Synthesis, and Spectroscopic Investigation of Zinc Dodecakis(trifluoroethoxy)phthalocyanines Conjugated with DeoxyribonucleosidesFNR HREF="nss"> FN ID="nss"> Support was provided by JSPS KAKENHI (17350047, 17590087, and 16655035). N.S. thanks Fuji Photo Film Co., Ltd. for an Award in Synthetic Organic Chemistry (Japan).
Ultrahigh-Resolution Backbone Structure of Perdeuterated Protein GB1 Using Residual Dipolar Couplings from Two Alignment MediaFNR HREF="nss"> FN ID="nss"> G.B. receives a grant from the CEA. This work was supported by the EU through EU-NMR JRA3 and by the French Research Ministry through ANR NT05-4_42781 and SNF grant 31-61'757.00 to S.G.
Induction of Structure and Function in a Designed Peptide upon Adsorption on a Silica NanoparticleFNR HREF="nss"> FN ID="nss"> The silica particles were kindly provided by EKA Chemicals, Stenungsund, Sweden. This work was supported by a grant from the Swedish National Science Research Council to B.-H.J. (K5104-5999) and by a grant from the Knut and Alice Wallenberg Foundation to K.B.
Control of Main‐Chain Stiffness of a Helical Poly(phenylacetylene) by Switching On and Off the Intramolecular Hydrogen Bonding through Macromolecular Helicity Inversion
Control of Main-Chain Stiffness of a Helical Poly(phenylacetylene) by Switching On and Off the Intramolecular Hydrogen Bonding through Macromolecular Helicity InversionFNR HREF="nss"> FN ID="nss"> We are deeply grateful to Professor T. Sato (Osaka University) for his fruitful discussions.
Dancing on a Fullerene Surface: Isomerization of Y3N@(N-Ethylpyrrolidino-C80) from the 6,6 to the 5,6 RegioisomerFNR HREF="nss"> FN ID="nss"> This work was supported by the Spanish Ministry of Science and Technology (Project no. CTQ2005-06909-C02-01-BQU and the Ramón y Cajal Program (ARF)) and by the DURSI of the Generalitat de Catalunya (2005SGR-00104). Part of the computer resources (CPMD calculations) were provided by the Barcelona Supercomputer Center (BSC).
A New Catalytic Route for the Activation of sp-Hybridized Carbon-Hydrogen BondsFNR HREF="nss"> FN ID="nss"> Financial support from the Ministry of Science and Higher Education (Poland) (grants 3T09A 145 26 and PBZ-KBN 118-T09-17) is gratefully acknowledged.
Cationic Rare-Earth Polyhydrido Complexes: Synthesis, Structure, and Catalytic Activity for the cis-1,4-Selective Polymerization of 1,3-CyclohexadieneFNR HREF="nss"> FN ID="nss"> This work was partly supported by Grant-in-Aid for Scientific Research from the Ministry of Education, Culture, Sports, Science, and Technology of Japan.
Relativistic Functional Groups: Aryl Carbon-Gold Bond Formation by Selective Transmetalation of Boronic AcidsFNR HREF="nss"> FN ID="nss"> We thank Case Western Reserve University and the donors of the Petroleum Research Fund, administered by the American Chemical Society (grant 42312-G3 to T.G.G.) for support. The diffractometer was funded by NSF grant 0087210, the Ohio Board of Regents grant CAP-491, and Youngstown State University.
The Diagnostic Substrate Bicyclohexane Reveals a Radical Mechanism for Bacterial Cytochrome P450 in Whole CellsFNR HREF="nss"> FN ID="nss"> We thank Dr. Enrico Funhoff for advice with the cell-free extract methodology, Charlotte Lehmann for technical assistance, and FMC Corp. (Princeton, NJ) for access to GC-MS instrumentation. We thank the NSF for funding (CHE-0221978 to R.N.A. and J.T.G. through the Environmental Molecular Sciences Institute CEBIC at Princeton University; CHE-0116233 to R.N.A.), the Camille and Henry Dreyfus Foundation (R.N.A.), and the NIH (GM072506 to R.N.A., and GM036298 to J.T.G.).
Selective Platination of Modified Oligonucleotides and Duplex Cross-LinksFNR HREF="nss"> FN ID="nss"> This work was supported by funds from the Ministerio de Educación y Ciencia (grant no. CTQ2004-8275) and the Generalitat de Catalunya (grant no. 2005SGR-693 and Centre de Referència de Biotecnologia).
Redox Targeting of Insulating Electrode Materials: A New Approach to High-Energy-Density BatteriesFNR HREF="nss"> FN ID="nss"> We acknowledge financial support of this work by a CTI project (contract No. 7136.3 EPRP-IW). We thank Dr. H. Li at the Institute of Physics, Chinese Academy of Sciences, for the kind help of making the carbon-free LiFePO4 sample.
Chemo- and Regioselective Preparation and Reaction of a Kinetic Zinc Enolate Formed from a Thiol Ester and Bis(iodozincio)methaneFNR HREF="nss"> FN ID="nss"> This work was supported financially by the Japanese Ministry of Education, Science, Sports, and Culture and by the Chugai Pharmaceutical Co., Ltd.
trans Influences on Hypervalent Bonding of Aryl λ3-Iodanes: Their Stabilities and Isodesmic Reactions of Benziodoxolones and BenziodazolonesFNR HREF="nss"> FN ID="nss"> We gratefully acknowledge the Ministry of Education, Culture, Sports, Science, and Technology of Japan for financial support in the form of a grant.
De Novo Design and Synthesis of Helix-Turn-Helix Structure from Short and Robust Mixed Helices Derived from C-Linked Carbo-β-Amino AcidsFNR HREF="nss"> FN ID="nss"> IICT Communication No. 061012. V.S., K.N., and A.R.S. thank CSIR, New Delhi, for financial support.
Sequence-Specific DNA Binding by Noncovalent Peptide-Tripyrrole ConjugatesFNR HREF="nss"> FN ID="nss"> This work was supported by the Spanish MEC (SAF2004-01044). J.B.B. thanks the Spanish M.E.C. for a predoctoral fellowship and M.E.V. thanks the HSFP organization for their support with a Career Development Award (CDA0032-2005-C) and the Spanish MEC for a "Ramon y Cajal" contract. We also thank Prof. J. Benavente for access to radioactivity facilities.
Inverse Axial-Ligand Effects in the Activation of H2O2 and ROOH by an MnIII CorrolazineFNR HREF="nss"> FN ID="nss"> This research was supported by the NSF (CHE-0606614).
Polyol Synthesis through Hydrocarbon Oxidation: De Novo Synthesis of L-GalactoseFNR HREF="nss"> FN ID="nss"> Financial support was provided by the Henry Dreyfus Foundation, the University of Illinois (UIUC), the Merck Research Laboratories, and the NIH-NIGMS (GM076153). D.J.C. gratefully acknowledges the UIUC for Roger Adams and C. S. Marvel fellowships. We thank Prof. E. N. Jacobsen (Harvard University) and Dr. C. P. Stevenson (Merck) for a gift of oligomeric (R,R)-[(salen)CoIII]OTf catalyst and helpful advice on the Payne rearrangement, respectively. We thank Johnson Matthey for a generous gift of Pd(OAc)2. We are also grateful to M. S. Chen for checking our experimental procedure for the allylic oxidation reaction (Table 1, entry 7).
Is the Ferric Hydroperoxy Species Responsible for Sulfur Oxidation in Cytochrome P450s?FNR HREF="nss"> FN ID="nss"> The authors are grateful to Prof. S. Chapman (University of Edinburgh) for the P450BM3 clones used in this work.
High-Temperature-Stable Catalysts by Hollow Sphere EncapsulationFNR HREF="nss"> FN ID="nss"> We thank A. Dreier and B. Spliethoff for the TEM analysis. Funding by the DFG through SFB 558 and the Leibniz program, in addition to the basic funding provided by the MPG, is gratefully acknowledged.
Hydrogen Storage in the Giant-Pore Metal-Organic Frameworks MIL-100 and MIL-101FNR HREF="nss"> FN ID="nss"> The authors are grateful to Dr. A. Vimont and Pr. M. Daturi (LCS, Caen, France) for the preliminary in situ IR experiments. J.-S.C. would like to thank KRICT for supporting this work under the institutional research program.
A Versatile Ruthenium Catalyst for C&bond;C Bond Formation by C&bond;H Bond ActivationFNR HREF="nss"> FN ID="nss"> This work was supported by the Centre National de la Recherche Scientifique (CNRS). R.M. thanks the Ministère de l'Education et de la Recherche for a grant. R.C. thanks Rhodia-Silicone for financial support. We thank Dr. Gérard Mignani (Rhodia-Silicone) for fruitful discussions.
Heterogeneous Copper-in-Charcoal-Catalyzed Click ChemistryFNR HREF="nss"> FN ID="nss"> We are grateful to the NSF for financial support. Discussions with Professor Craig Hawker and his group (UCSB) are warmly acknowledged. ICP-AES analyses were conducted by Anthony E. Tomaso (UCSB) and are much appreciated.
Eine neue nicht-zentrosymmetrische Modifikation von BiB3O6FNR HREF="nss"> FN ID="nss"> Wir danken der DFG für die großzügige Unterstützung (HU 966-2-2), Dr. P. Mayer für die Datensammlung am Einkristall, T. Miller für die temperaturabhängigen Pulverbeugungsdaten, Dr. L. Bayarjargal für seine Hilfe bei den SHG-Messungen sowie Prof. Dr. L. Bohatý (Universität zu Köln) und Prof. Dr. W. Schnick (LMU München) für Ihre Unterstützung.
Goldkatalysatoren: Nanoporöse Gold-SchwämmeFNR HREF="nss"> FN ID="nss"> Für finanzielle Unterstützung danken wir dem Fonds der Chemischen Industrie. Diese Arbeit wurde zum Teil mit Unterstützung des U.S. Department of Energy an der University of California, Lawrence Livermore Laboratory unter der Vertragsnummer W-7405-Eng-48 durchgeführt. Für hilfreiche Diskussionen danken wir Prof. Dr. Günter Schulz-Eckloff.
α- und β-[Fe2(µ-StBu)2(StBu)4]2- - Koexistenz zweier Bindungsdehnungsisomere einer klassischen bitetraedrischen Metall-Chalkogenolat-VerbindungFNR HREF="nss"> FN ID="nss"> Diese Arbeit wurde von der Deutschen Forschungsgemeinschaft (DFG), vom Bundesministerium für Bildung, Wissenschaft, Forschung und Technologie (BMBF) und vom Fonds der Chemischen Industrie unterstützt.