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Titelbild: Achieving Molecular Complexity by Organocatalytic One-Pot Strategies-A Fast Entry for Synthesis of Sphingoids, Amino Sugars, and Polyhydroxylated a-Amino Acids (Angew. Chem. 37/2009)
Jiang, H.
/ Elsner, P.
/ Jensen, K. L.et al.
| 2009
Titelbild: Achieving Molecular Complexity by Organocatalytic One‐Pot Strategies—A Fast Entry for Synthesis of Sphingoids, Amino Sugars, and Polyhydroxylated α‐Amino Acids (Angew. Chem. 37/2009)
Zur Biosynthese von Thiopeptidantibiotika Unsere Arbeiten wurden von der DFG (Emmy Noether-Nachwuchsgruppe an H.-D. A.) und dem FCI gefördert. S.S. und J.-Y.L. sind Mitglieder der IMPRS-CB. Wir danken Prof. Rolf Müller (Universität Saarbrücken) und Dr. Mark Brönstrup (Sanofi-Aventis, Frankfurt a. M.) für Diskussionen.
Efficient Regeneration of Partially Spent Ammonia Borane Fuel This work was funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy. We would like to thank Drs. Troy Semelsberger and Roshan Shrestha for GC characterization of H2 released during digestion. D.A.D. thanks the Robert Ramsay Fund at the University of Alabama for partial support.
Boron Mimetics: 1,2-Dihydro-1,2-azaborines Bind inside a Nonpolar Cavity of T4 Lysozyme The authors thank Dr. Walter A. Baase for his helpful comments and discussion. Support has been provided by the University of Oregon and NIH grant GM21967. The authors also thank Drs. Derek Yoder and Craig Ogata at Beamline IB-23-D, Advanced Photon Source, and Drs. Jeff Dickert and Peter Zwart at Beamline 5.0.2, Advanced Light Source, for their help in data collection.
Substrate-Assisted Assembly of Interconnected Single-Duplex DNA Nanostructures We thank Dr. Paul W. K. Rothemund and Prof. Sung Ha Park for helpful suggestions and discussions, and Rizal F. Hariadi for help in the early stages of the experiments. This work is supported by a Grant-in-Aid for Scientific Research (A) 19200023 and The Mitsubishi Foundation (2007) (S.M.), and JSPS Research Fellowships for Young Scientists (no. 21-8655) to S.H.
Synthesis of Out-of-Substrate Au-Ag Nanoplates with Enhanced Stability for Catalysis The submitted manuscript was created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a US Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The US Government retains for itself, and others acting on its behalf, a paid-up, nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. Use of the Center for Nanoscale Materials and the Electron Microscopy Center for Materials Research at Argonne was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Characterizations were also carried out by partially using the Center for Microanalysis of Materials Facilities in Frederick Seitz Materials Research Laboratory, University of Illinois, which is partially supported by the US Department of Energy under Grant No. DEFG02-91-ER45439.
Monitoring Protein Kinases in Cellular Media with Highly Selective Chimeric Reporters We thank Prof. K. A. Dalby for valuable advice and for providing DNA of the PNT domain and the PEA-15 protein, and Dr. Kevin Janes for helpful discussions. This research was supported by the NIH Cell Migration Consortium (GM064346). The Biophysical Instrumentation Facility for the Study of Complex Macromolecular Systems (NSF-0070319) is also gratefully acknowledged.
Dilution-Free Analysis from Picoliter Droplets by Nano-Electrospray Ionization Mass Spectrometry This research was supported by the U.S. D.O.E. Office of Biological and Environmental Research, the NIH NCRR (RR018522), the National Institute of Allergy and Infectious Diseases, and the WA State Life Sciences Discovery Fund. Microfabrication and experimental work were performed in the PNNL Environmental Molecular Sciences Laboratory.
Recycling the Waste: The Development of a Catalytic Wittig Reaction We thank The University of Texas at Arlington (UTA) for funding this work and ThalesNano (Hungary) for their collaborative in-kind donation (in part) of an H-Cube Midi used to synthesize 1. C.J.O.B. thanks Prof. Daniel W. Armstrong and Edra Dodbiba for separation of 1. G.A.C. thanks GIOCOMMS for computational resources and CAFMaD (Wales (UK)) for personal support.
Unusual Allylpalladium Carboxylate Complexes: Identification of the Resting State of Catalytic Enantioselective Decarboxylative Allylic Alkylation Reactions of Ketones We thank NIH-NIGMS (R01 GM 080269-01), Abbott Laboratories, Amgen, Merck, Bristol-Myers Squibb, Boehringer Ingelheim, the Fannie and John Hertz Foundation (predoctoral fellowship to DCB), the Gordon and Betty Moore Foundation, and Caltech for financial support. Lawrence Henling and Dr. Michael Day are gratefully acknowledged for X-ray crystallographic structural determination. The Bruker KAPPA APEX II X-ray diffractometer was purchased through an NSF CRIF:MU award to the California Institute of Technology, CHE-0639094. Prof. J. E. Bercaw, Prof. R. H. Grubbs, Prof. S. E. Reisman, Prof. W. A. Goddard III, and Dr. J. A. Keith are acknowledged for helpful discussions. Dr. David Vander Velde and Dr. Scott Ross are thanked for helpful assistance related to NMR.
Unusual Allylpalladium Carboxylate Complexes: Identification of the Resting State of Catalytic Enantioselective Decarboxylative Allylic Alkylation Reactions of Ketones
Sherden, Nathaniel H.
/ Behenna, Douglas C.
/ Virgil, Scott C.et al.
| 2009
Achieving Molecular Complexity by Organocatalytic One‐Pot Strategies—A Fast Entry for Synthesis of Sphingoids, Amino Sugars, and Polyhydroxylated α‐Amino Acids
Achieving Molecular Complexity by Organocatalytic One-Pot Strategies-A Fast Entry for Synthesis of Sphingoids, Amino Sugars, and Polyhydroxylated α-Amino Acids This work was made possible by a grant from The Danish National Research Foundation, OChemSchool, and the Carlsberg Foundation.
Achieving Molecular Complexity by Organocatalytic One-Pot Strategies-A Fast Entry for Synthesis of Sphingoids, Amino Sugars, and Polyhydroxylated a-Amino Acids
Jiang, H.
/ Elsner, P.
/ Jensen, K. L.et al.
| 2009
Ultrasensitive and Selective Colorimetric DNA Detection by Nicking Endonuclease Assisted Nanoparticle Amplification We acknowledge the DSTA (R-143-000-379), Singapore-MIT Alliance, and A*STAR (SERC 082-101-0026) for supporting this work. X.L. is grateful to the National University of Singapore for a Start-Up Grant Award (R-143-000-317) and a Young Investigator Award (R-143-000-318).
Cobalt(II)-Responsive DNA Binding of a GCN4-bZIP Protein Containing Cysteine Residues Functionalized with Iminodiacetic Acid This research was supported in part by Grants-in-Aid for Scientific Research from the Ministry of Education, Culture, Sports, Science, and Technology of Japan. Y.A. is grateful for a JSPS Research Fellowship for Young Scientists.
Absolute Asymmetric Reduction Based on the Relative Orientation of Achiral Reactants This research was supported by the Rowland Institute at Harvard and the French Ministry of Education and Research. We are grateful to Gary Widiger, Chris Stokes, Don Rogers, Doug Ho, Michelle Li, and Jim Foley for technical support and helpful discussions.
Large-Scale Soft Colloidal Template Synthesis of 1.4 nm Thick CdSe Nanosheets This work was supported by the National Research Foundation of Korea (NRF) through the National Creative Research Initiative Program and by NSF Research Grant CHE-0613306 (R.H.).
Highly Selective CO2 Capture in Flexible 3D Coordination Polymer Networks This work was supported by a Korea Research Foundation Grant (Basic Research Promotion Fund, KRF-2005-084-C00020), and by the SRC program of MOST-KOSEF through the Center for Intelligent Nano-Bio Materials (grant: R11-2005-008-00000-0).
Total Synthesis of Hirsutellone B We gratefully acknowledge financial support from the National Institutes of Health (USA), National Science Foundation (CHE-0603217), Natural Sciences and Engineering Research Council, Canada (postdoctoral fellowship to T.R.W.) and Skaggs Institute for Research. We thank Dr. M. Isaka and Prof. Y. Thebtaranonth for NMR spectra of natural hirsutellone B.
Bis(σ-amine-borane) Complexes: An Unusual Binding Mode at a Transition-Metal Center The authors thank the EPSRC and University of Oxford for support. Dedicated to Professor Jennifer Green on the occasion of her retirement.
A General and Mild Palladium-Catalyzed Domino Reaction for the Synthesis of 2H-Indazoles We thank D. I. W. Heyse, H. Schweitzer, and Dr. N. Nagel for solving the X-ray crystal structure. This research was supported by the European Community through a Marie Curie Host Fellowship for the Transfer of Knowledge (HCTMCR).
Controllable Polyol Synthesis of Uniform Palladium Icosahedra: Effect of Twinned Structure on Deformation of Crystalline Lattices This work was supported by Grant-in-Aid for Scientific Research on Priority Area "Strong Photon-Molecule Coupling Fields for Chemical Reactions" (No. 470)(19049007). C.L. and R.S. acknowledge the JSPS Postdoctoral Fellowship for Foreign Researchers (1907354) and the JSPS Research Fellowship for Young Scientists (20685), respectively.
Polymer-Functionalized Platinum-On-Gold Bimetallic Nanorods This work was supported by the NSF CAREER Award (DMR-0547399), Robert A. Welch Foundation (C-1703), and Alfred Sloan Foundation.
Palladium-katalysierte Amidierung nichtaktivierter C(sp3)-H- Bindungen: von Anilinen zu Indolinen Wir danken der Deutschen Forschungsgemeinschaft, dem Fonds der Chemischen Industrie (Stipendium für J.J.N.) und der International NRW Graduate School of Chemistry (Stipendium für S.R.) für großzügige finanzielle Unterstützung. Die Forschung von F.G. wird gefördert durch den Alfried Krupp-Preis für junge Hochschullehrer der Alfried Krupp von Bohlen und Halbach-Stiftung. N. Kuhl und M. Pawelczyk danken wir für die Herstellung einiger Startmaterialien.
Biomimetische Lipo-Glycopolymer-Membranen: photochemische Oberflächenanbindung supramolekularer Architekturen mit definierter Orientierung Wir danken Dr. Tobias Baumgart und Dr. M. Sever für hilfreiche Diskussionen sowie dem FRIAS, dem Rektorat der Universität Freiburg und dem MPIP für ihre Unterstützung.
Hochauflösende Mikroskopie mit kleinen organischen Farbstoffen Diese Arbeit wurde durch die Forschungsschwerpunkte Biophotonik und Systembiologie (FORSYS) des Bundesministeriums für Bildung und Forschung (BMBF, Nr. 13N9234 und 0315262) unterstützt.
Feste Katalysatoren für die selektive Niedertemperaturoxidation von Methan zu Methanol Diese Arbeit wurde im Rahmen des Projekthauses "ENERCHEM" der Max-Planck-Gesellschaft angefertigt. Wir danken B. Spliethoff (MPI für Kohlenforschung) für TEM- und S. Palm für REM-Messungen sowie Dr. C. Weidenthaler für XRD- und XPS-Untersuchungen und hilfreiche Diskussionen.
Heteroatome steigern die Selektivität der oxidativen Dehydrierung an Nanokohlenstoff Diese Arbeit wurde vom EnerChem-Projekt (Max-Planck-Gesellschaft) gefördert. Die Autoren danken Prof. R. Schomäcker (Technische Universität Berlin), E. Kitzelmann, G. Weinberg, Dr. D. Rosenthal und Dr. Bo Zhu für experimentelle Unterstützung und hilfreiche Diskussionen.