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Titelbild: Enantiogruppen-differenzierende intramolekulare Aldolisierung durch Katalyse mit einem primaren Amin (Angew. Chem. 40/2008)
Mechanismus der schnellen Peptiderkennung durch SH3-Domänen M.A. dankt der Tishreen-Universität (Syrien) für ein Promotionsstipendium. Dieses Projekt wurde teilweise durch die Volkswagenstiftung gefördert (Projekt I-80469).
Europium-basierte ionische Flüssigkeiten als lumineszierende weiche Materialien Dank gilt der DFG für Unterstützung im Rahmen des Schwerpunktprogrammes "Lanthanoidspezifische Funktionalitäten" SPP 1191. A.V.M. dankt dem Fonds der Chemischen Industrie für ein Chemiedozenten-Stipendium.
Bei Raumtemperatur flüssige ionische Verbindungen auf Dysprosium-Basis mit starker Lumineszenz und Reaktion auf magnetische Felder Dank gilt der DFG für Unterstützung im Rahmen des Schwerpunktprogrammes "Lanthanoidspezifische Funktionalitäten" SPP 1166. A.V.M. dankt dem Fonds der Chemischen Industrie für ein Chemiedozenten-Stipendium.
Imidazoliumbasierte ionische Flüssigkeiten als effiziente forminduzierende Lösungsmittel für die Synthese von Gold-Nanostäbchen Diese Arbeit wurde von der Deutschen Forschungsgemeinschaft (Bo 1948-1-2), der National Science Foundation (DMR-0351770 und DMR-0706265) und dem INTEL IFYRE Programm (A.R.) gefördert. Wir danken Tom Nuhfer für seine Hilfe bei der hochauflösenden Transmissionselektronenmikroskopie.
Regulation der Aktivität von humaner Carboanhydrase I (hCAI) durch einen photochromen Inhibitor Diese Arbeit wurde von der Deutschen Forschungsgemeinschaft, dem Fonds der chemischen Industrie, der Universität Regensburg, dem Natural Sciences and Engineering Research Council of Canada, dem Canada Research Chair Program und der Simon Fraser University unterstützt.
Synthese von Aryl- und Heteroarylindium(III)-Verbindungen durch direkte Insertion von Indium in Gegenwart von LiCl Y.-H.C. dankt der Alexander von Humboldt-Stiftung für die finanzielle Unterstüzung. Wir danken dem Fonds der Chemischen Industrie, der DFG, der Chemetall GmbH (Frankfurt) und der BASF AG (Ludwigshafen) für die finanzielle Unterstützung.
Iridiumkatalysierte asymmetrische allylische Substitutionen - sehr hohe Regioselektivitat und Luftstabilitat mit einem Katalysator auf der Basis von Dibenzo[a,e]cyclooctatetraen und einem Phosphoramidit
Iridiumkatalysierte asymmetrische allylische Substitutionen - sehr hohe Regioselektivität und Luftstabilität mit einem Katalysator auf der Basis von Dibenzo[a,e]cyclooctatetraen und einem Phosphoramidit Diese Arbeit wurde vom Fonds der Chemischen Industrie, der Deutschen Forschungsgemeinschaft (SFB 623) und der Landesgraduiertenförderung unterstützt. Wir danken Dr. F. Rominger für die Röntgenkristallstrukturanalyse. Dank der Unterstützung durch ein IJP-Stipendium der Royal Society für Dr. J. M. Brown und G.H. konnten NMR-spektroskopische Untersuchungen von C.W. während mehrerer Besuche in Oxford vorgenommen werden. Wir danken Dr. Brown und seinen Mitarbeitern für ihre großzügige Hilfe und fruchtbare Diskussionen.
Iridiumkatalysierte asymmetrische allylische Substitutionen – sehr hohe Regioselektivität und Luftstabilität mit einem Katalysator auf der Basis von Dibenzo[a,e]cyclooctatetraen und einem Phosphoramidit
Enantiogruppen-differenzierende intramolekulare Aldolisierung durch Katalyse mit einem primären Amin Wir danken der Max-Planck-Gesellschaft, der DFG (Schwerpunktprogramm "Organokatalyse" SPP1179), dem Fonds der Chemischen Industrie und der Wacker Chemie AG für ihre großzügige Unterstützung.
Totalsynthese von natürlich konfiguriertem Pyrrhoxanthin, einem Carotinoid-Butenolid aus Plankton Wir danken der Deutschen Forschungsgemeinschaft für die Förderung dieses Projekts und Dr. Thomas Netscher (DSM Nutritional Products, Basel) für mehrere Spenden von (-)-Actinol.
C1-Symmetric Monosubstituted Chiral Diene Ligands in Asymmetric Rhodium-Catalyzed 1,4-Addition Reactions This work was support by the Centre National de la Recherche Scientifique (CNRS). T. Gendrineau thanks the Ministère de l'Education et de la Recherche for a grant.
Synthesis of Biaryl Compounds through Three‐Component Assembly: Ambidentate Effect of the tert‐Butyldimethylsilyl Group for Regioselective Diels–Alder and Hiyama Coupling Reactions
Synthesis of Biaryl Compounds through Three-Component Assembly: Ambidentate Effect of the tert-Butyldimethylsilyl Group for Regioselective Diels-Alder and Hiyama Coupling Reactions This work was supported by Grants-in-Aid for Scientific Research and the global COE program from the Ministry of Education, Culture, Sports, Science, and Technology (Japan). We thank the Uehara Memorial Foundation for financial support.
Synthetic Scheme for High-Quality InAs Nanocrystals Based on Self-Focusing and One-Pot Synthesis of InAs-Based Core-Shell Nanocrystals X. Peng thanks the NSF and NIH for funding support, and we thank Dr. M. Benamara for HRTEM measurements.
Spontaneous Growth of Highly Conductive Two-Dimensional Single-Crystalline TiSi2 Nanonets This work was financially supported by Boston College. We are grateful to Prof. J. Kong and Y.-P. Hsieh at MIT for their generous help in carrying out Raman experiments. E. Shaw at MIT provided assistance in XPS experiments. Dr. D. Wang helped with TEM.
Hollow Spheres to Nanocups: Tuning the Morphology and Magnetic Properties of Single-Crystalline α-Fe2O3 Nanostructures We thank the IISc Nanoinitiative for use of the Technai TEM instrument and N. R. Selvi of JNCASR for FESEM measurements. U.M. thanks JNCASR for a Summer Research Fellowship.
Rate and Selectivity Enhancements Mediated by OH Radicals in the Oxidative Coupling of Methane Catalyzed by Mn-Na2WO4-SiO2 This study was supported by BP as part of the Methane Conversion Cooperative Research Program at the University of California at Berkeley.
Intermolecular Hydroarylation of Unactivated Olefins Catalyzed by Homogeneous Platinum Complexes We thank the National Science Foundation (CHE-0137394 and CHE-0719372) for financial support, Dr. W. Kaminsky and Dr. J. Benedict for performing the X-ray structural determinations and Prof. K. McNeill (University of Minnesota) for initial samples of the ligand 3.
Bioinspired Dismutation of Chlorite to Dioxygen and Chloride Catalyzed by a Water-Soluble Iron Porphyrin This research was supported by a grant from the US National Science Foundation (CHE-0749572). We thank Dr. Katya Albert, Prof. Dale Margerum, Chelsea Thompson, and Prof. Paul Shepson for assistance with IC. We thank Alan Ronemus for design and implementation of RGA. We thank Dr. Guodong Du for assistance with translation of a Chinese manuscript. Lastly, we thank Prof. Hilkka Kentämaa and Mr. Stephen Habicht for assistance with ESI-MS on 18O-enriched NaClO2.
Agostic NSi&bond;H···Mo Complexes: From Curiosity to Catalysis This work was supported by the Petroleum Research Fund, administered by the American Chemical Society. L.G.K. thanks the Russian Foundation of Basic Research.
Tunable Molecular Assembly Codes Direct Reaction Pathways We acknowledge support from the National Institute of General Medicine Sciences (Grant GM065306), the Mass Spectrometry Core Laboratories at WSU for discussions concerning MALDI data, and the WSU Center for NMR spectroscopy for assistance with variable temperature NMR studies. A.D.Q.L. is a former Beckman Young Investigator (BYI).
Asymmetric Aza-Michael Reactions of α,β-Unsaturated Ketones with Bifunctional Organic Catalysts We are grateful for financial support from theNational Institute of Health (GM-61591).
Modularly Designed Organocatalytic Assemblies for Direct Nitro-Michael Addition Reactions We thank the Welch Foundation (Grant No. AX-1953) for the financial support of this project.
Enantioselective Cu-Catalyzed 1,4-Addition of Grignard Reagents to Cyclohexenone Using Taddol-Derived Phosphine-Phosphite Ligands and 2-Methyl-THF as a Solvent This work was carried out in the context of Cost D40 and supported by the European Commission (Ligbank), the Chemetall GmbH, and the Fonds der Chemischen Industrie.
Enantioselective Cu‐Catalyzed 1,4‐Addition of Grignard Reagents to Cyclohexenone Using Taddol‐Derived Phosphine–Phosphite Ligands and 2‐Methyl‐THF as a Solvent
Surfactant-Assisted Synthesis of Nanoscale Gadolinium Metal-Organic Frameworks for Potential Multimodal Imaging We acknowledge financial support from NSF and NCI. We thank W. J. Rieter and Dr. L. Ma for experimental help.
Trimodular Engineering of Linear Supramolecular Miniatures on Ag(111) Surfaces Controlled by Complementary Triple Hydrogen Bonds This work was financially supported by the EU RTN PRAIRIES, contract MRTN-CT-2006-035810, MIUR (Firb RBIN04HC3S), the SNSF, the NCCR "Nanoscale Science" in Basel, the Belgian National Research Foundation (FRS-FNRS, through the contract No. 2.4.625.08 F), and the University of Namur. A.L.P. thanks the University of Trieste for the doctoral fellowship. We also thank the Swiss Federal Commission for Technology and Innovation, KTI, and Nanonis Inc. for the fruitful collaboration on the data acquisition system.
Tuning of Electrogenerated Silole Chemiluminescence This work was supported by NSERC, PREA, CFI, OIT, and UWO. We thank FMC Lithium, a division of FMC Corporation, for a generous donation of tBu2Si(OTf)2, and we thank Lindsay Kelland for ECL experiments.
Crystallography-Independent Determination of Ligand Binding Modes This work was supported by the Volkswagen-Stiftung (grant to T.C.), the Fonds der chemischen Industrie (fellowship no. 180081 to J.O.; support to C.G.), the Max-Planck Gesellschaft, and Sanofi-Aventis. We thank Elke Duchardt for the measurement of some interligand NOE spectra, Sandra Schimanski-Breves for crystallization, Thomas Langer for protein production of Chinese hamster protein kinase A (PKA), and Prof. H. Schwalbe for the provision of previously reported expression plasmids. Bovine PKA was obtained from Dirk Bossemeyer and Michael Gassel. Crystallographic data were collected on beamline ID14.1 at the European Synchotron Radiation Facility (ESRF).
A Comparison of the H2 Sorption Capacities of Isostructural Metal-Organic Frameworks With and Without Accessible Metal Sites: [{Zn2(abtc)(dmf)2}3] and [{Cu2(abtc)(dmf)2}3] versus [{Cu2(abtc)}3] This work was supported by a Korea Research Foundation Grant funded by the Korean Government (MOEHRD, Basic Research Promotion Fund; grant no. KRF-2005-084-0C00020) and by the Korea Science and Engineering Foundation (grant KOSEF, R11-2005-008-00000-0), Republic of Korea. H4abtc=1,1'-azobenzene-3,3',5,5'-tetracarboxylic acid.
A Comparison of the H2 Sorption Capacities of Isostructural Metal–Organic Frameworks With and Without Accessible Metal Sites: [{Zn2(abtc)(dmf)2}3] and [{Cu2(abtc)(dmf)2}3] versus [{Cu2(abtc)}3]
Lee, Yong‐Gon
/ Moon, Hoi Ri
/ Cheon, Young Eunet al.
| 2008
Sources of Error in DFT Computations of C&bond;C Bond Formation Thermochemistries: π→σ Transformations and Error Cancellation by DFT Methods We are grateful to the National Science Foundation and the Partnerships for Advanced Computational Infrastructure (PACI) for the financial support of this research. The computations were performed on the UCLA Academic Technology Services (ATS) Hoffman Beowulf cluster.
Controlled Synthesis of Photomagnetic Nanoparticles of a Prussian Blue Analogue in a Silica Xerogel This research was supported by the French Government through the ANR "Blue Memory" (BLAN06-3_134929). We would also like to thank E. Rivière (ICMMO-ECI) for SQUID measurements and P. Beaunier (Service de microscopie électronique, Université Pierre et Marie Curie) for TEM studies.
Diffusively Coupled Chemical Oscillators in a Microfluidic Assembly This work was supported by the National Science Foundation (CHE-0615507) and the Defense Advanced Research Projects Agency. We thank Milos Dolnik and Anatol Zhabotinsky for helpful comments and suggestions.
Ribosomal Synthesis of Tricyclic Depsipeptides in Bloom-Forming Cyanobacteria We thank M.-G. Schwinger for E. coli mass culture, Dr. R. Winkler and M. Pötsch for MALDI-TOF analyses, A. Perner for HRMS and HPLC-MS measurements, R. Günther, K. Hinrichs, and J. Müller for their assistance with the molecular work, and U. Newen, Leibniz-Institute for Freshwater Ecology and Inland Fisheries, Berlin. Financial support by the Leibniz Gemeinschaft, the DFG (ILRS, JSMC, SPP1152) and the German-Israeli Foundation (GIF) is gratefully acknowledged.
An Electron-Transfer Ferromagnet with Tc=107 K Based on a Three-Dimensional [Ru2]2-TCNQ System This work was supported by a Grant-in-Aid for Scientific Research from the Ministry of Education, Culture, Sports, Science, and Technology (Japan) and The Asahi Glass Foundation (H.M.). K.R.D. thanks the National Science Foundation Chemistry Division for financial support.
Activation of Protein Splicing by Protease- or Light-Triggered O to N Acyl Migration We thank Prof. D. Raleigh and H. Taskent for access to stop-flow and circular dichroism instruments and to them and E. George for helpful discussions. This work was supported by NIH grants EB001991 and GM55843 to T.W.M. M.V.P. and M.R. were supported by the Spanish Ministry of Science and Education.