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3067
Cover Picture: Carboxylic Acids as Substrates in Homogeneous Catalysis (Angew. Chem. Int. Ed. 17/2008)
Polymer-Induced Transient Pores in Lipid MembranesFNR HREF="nss"> FN ID="nss"> We kindly acknowledge a grant from the FWF 18740B03 for financial support.
Shaping of a Conformationally Flexible Molecular Structure for SpectroscopyFNR HREF="nss"> FN ID="nss"> This work was supported by the EU projects Hy3M and STAG as well as the Netherlands Organization for Scientific Research (NWO).
METAMORPhos: Adaptive Supramolecular Ligands and Their Mechanistic Consequences for Asymmetric HydrogenationFNR HREF="nss"> FN ID="nss"> The NRSC-C, BASF, and EZ are acknowledged for financial support, Dr. P. A. Breuil for providing ligand 3, Dr. J. M. Ernsting and Dr. J. Geenevasen for assistance with the NMR experiments, and Dr. H. Peeters for the mass spectrometry experiments.
The Direct Conversion of Light into Continuous Mechanical Energy by Photoreversible Self-Assembly: A Prototype of a Light-Powered EngineFNR HREF="nss"> FN ID="nss"> We thank Profs. G. Gottarelli and C. Zannoni (Bologna) for helpful discussions and suggestions. Thanks are also due to Dr. M. A. Cremonini and Prof. G. Placucci for their kind hospitality at the NMR facility, Campus di Scienze degli Alimenti (Forlì-Cesena). Technical assistance by G. Gnudi (F.A.V.S. Scientific Glassworks, Bologna) is gratefully acknowledged. Financial support was provided by MiUR (PRIN Projects) and the University of Bologna.
A Straightforward Route to Helically Chiral N‐Heteroaromatic Compounds: Practical Synthesis of Racemic 1,14‐Diaza[5]helicene and Optically Pure 1‐ and 2‐Aza[6]helicenes
Míšek, Jiří
/ Teplý, Filip
/ Stará, Irena G.et al.
| 2008
A Straightforward Route to Helically Chiral N-Heteroaromatic Compounds: Practical Synthesis of Racemic 1,14-Diaza[5]helicene and Optically Pure 1- and 2-Aza[6]helicenesFNR HREF="nss"> FN ID="nss"> This research was supported by the European Commission under Grant No. FP6-015847 and by the Grant Agency of the Czech Republic under Grant No. 203-06-1792.
Phototriggering of Cell Adhesion by Caged Cyclic RGD PeptidesFNR HREF="nss"> FN ID="nss"> We thank Neo MPS Laboratories (Strasbourg, France) for synthesizing the peptide, and Alexandra Goldyn, Henriette Ries, and Ralf Kemkemer (research group of Prof. J. Spatz, MPI für Metallforschung, Stuttgart, Germany) for help with the cell experiments. The RGD peptide sequence is Arg-Gly-Asp.
A Portable Albumin Binder from a DNA-Encoded Chemical LibraryFNR HREF="nss"> FN ID="nss"> We thank Miljen Martic for help with the HPLC analysis of radioactive derivatives, Madalina Jaggi for help with the synthesis of the DNA-encoded chemical library, and Dr. Jens Sobek and Dr. Ralph Schlapbach (Functional Genomics Center Zurich) for the microarrays. Financial support from ETH Zürich, Philochem AG, the Swiss National Science Foundation, Bundesamt für Bildung und Wissenschaft (EU Project STROMA), the EU FP6 Projects Immuno-PDT and DIANA, the German Research Council DFG (Se837-4-1 and 5-1 to M.W.S.), and IP "EVI-GenoRet" LSHG-CT-512036 (to M.W.S.) is gratefully acknowledged.
Effects of Guanidinium–Phosphate Hydrogen Bonding on the Membrane‐Bound Structure and Activity of an Arginine‐Rich Membrane Peptide from Solid‐State NMR Spectroscopy
Tang, Ming
/ Waring, Alan J.
/ Lehrer, Robert I.et al.
| 2008
Synthesis of an Extremely Bent Acyclic Allene (A "Carbodicarbene"): A Strong Donor LigandFNR HREF="nss"> FN ID="nss"> We are grateful to the NSF (CHE 0518675) for financial support of this work, the NSERC for a postdoctoral fellowship (C.A.D.), and the ACS for a graduate fellowship (V.L.).
Coordination Chemistry of Ene-1,1-diamines and a Prototype "Carbodicarbene"FNR HREF="nss"> FN ID="nss"> Financial support by the MPG, the Spanish Ministerio de Educación y Ciencia (fellowship to M.A.), and the Fonds der Chemischen Industrie is gratefully acknowledged. We thank Umicore AG & Co KG, Hanau, for the generous gift of noble-metal salts.
The Use of Single-Source Precursors for the Solution-Liquid-Solid Growth of Metal Sulfide Semiconductor NanowiresFNR HREF="nss"> FN ID="nss"> We thank the National Science Foundation (grant no. CHE-0518427) for support of this work, and Richard A. Loomis and John G. Glennon for assistance with NIR spectroscopy.
Aerobic Alcohol Oxidation Coupled to Palladium-Catalyzed Alkene Hydroarylation with Boronic EstersFNR HREF="nss"> FN ID="nss"> This work was supported by the National Institutes of Health (Grant NIGMS RO1 GM3540). M.S.S. thanks the Dreyfus Foundation (Teacher-Scholar) and Pfizer for their support. Y.I. thanks Kyorin Co., Ltd. for financial support. K.M.G. thanks Sanofi-Aventis for a graduate research fellowship. We are grateful to Johnson Matthey for the gift of various Pd salts.
Transfer Semihydrogenation of Alkynes Catalyzed by a Zero-Valent Palladium N-Heterocyclic Carbene ComplexFNR HREF="nss"> FN ID="nss"> This research was funded by the National Research School Combination Catalysis (project no. 2004-2008-UVA-Elsevier-02-03). G.M. was the recipient of a Socrates-Erasmus fellowship from the University of Parma. We thank Dr. G. Rothenberg for helpful discussions and a critical reading of the manuscript.
Catalytic Abatement of Nitrous Oxide Coupled with Selective Production of Hydrogen and EthyleneFNR HREF="nss"> FN ID="nss"> This work was partially supported by the DFG (Deutsche Forschungsgemeinschaft) within the collaborative research center (Sonderforschungsbereich) 546.
A Heterobimetallic Pd-La-Schiff Base Complex for anti-Selective Catalytic Asymmetric Nitroaldol Reactions and Applications to Short Syntheses of β-Adrenoceptor AgonistsFNR HREF="nss"> FN ID="nss"> This work was partially supported by a Grant-in-Aid for Specially Promoted Research from MEXT, and a Grant-in-Aid for Encouragements for Young Scientists (B) (Y.S.), from JSPS, and Mitsubishi Chemical Corporation Fund (S.M.), and Toray Co Ltd.
A Heterobimetallic Pd/La/Schiff Base Complex for anti‐Selective Catalytic Asymmetric Nitroaldol Reactions and Applications to Short Syntheses of β‐Adrenoceptor Agonists
Enantioselective Synthesis of an Atropisomeric Diaryl EtherFNR HREF="nss"> FN ID="nss"> We are grateful to the EPSRC and GlaxoSmithKline for support, and to Dr. Simon Peace for helpful discussions.
Enantioselective Phase-Transfer-Catalyzed Intramolecular Aza-Michael Reaction: Effective Route to Pyrazino-Indole CompoundsFNR HREF="nss"> FN ID="nss"> Acknowledgements are made to the MIUR (Rome), Consorzio C.I.N.M.P.I.S., and University of Bologna. We kindly thank Dr. Paolo Melchiorre (University of Bologna) for helpful discussions.
Total Synthesis of (+)-Neopeltolide by a Prins MacrocyclizationFNR HREF="nss"> FN ID="nss"> This work was supported by a grant from MarineBio21, Ministry of Maritime Affairs and Fisheries, Korea, and a grant from the Center for Bioactive Molecular Hybrids (Yonsei University and KOSEF). BK21 graduate fellowship grants to M.S.K. are gratefully acknowledged.
Ethanol as Hydrogen Donor: Highly Efficient Transfer Hydrogenations with Rhodium(I) AmidesFNR HREF="nss"> FN ID="nss"> This work was supported by the Swiss National Science Foundation (SNF) and the ETH Zürich.
Dichotomic Reactivity of a Stable Silylene toward Terminal Alkynes: Facile C&bond;H Bond Insertion versus Autocatalytic Formation of Silacycloprop-3-eneFNR HREF="nss"> FN ID="nss"> Financial support from the Deutsche Forschungsgemeinschaft and the Cluster of Excellence "Unifying Concepts in Catalysis" (EXC 314-1) are gratefully acknowledged.
The Complete Stereochemistry of the Enzymatic Dehydration of 4-Hydroxybutyryl Coenzyme A to Crotonyl Coenzyme AFNR HREF="nss"> FN ID="nss"> We thank Ulrike Näser (Newcastle University) for devising the synthetic route to succinic acid semialdehyde, Thomas Knappe, Professor Mohammed Marahiel (both at Philipps-Universität Marburg), Simone Moser, and Professor Bernhard Kräutler (both at Universität Innsbruck, Austria) for measuring the CD spectra, as well as Professor James Remington (University of Oregon (USA)) for sending the plasmid with the malate synthase gene. The Deutsche Forschungsgemeinschaft, the European Commission (Contract HPRN-CT-2002-00195), and the Fonds der Chemischen Industrie funded this work.
Proximicins A, B, and C—Antitumor Furan Analogues of Netropsin from the Marine Actinomycete Verrucosispora Induce Upregulation of p53 and the Cyclin Kinase Inhibitor p21
Proximicins A, B, and C-Antitumor Furan Analogues of Netropsin from the Marine Actinomycete Verrucosispora Induce Upregulation of p53 and the Cyclin Kinase Inhibitor p21FNR HREF="nss"> FN ID="nss"> The work was supported by the DFG (project SU 239-5-1) and from the European Commission (project ACTINOGEN, 6th framework, LSHM-CT-2004-005224). We thank G. Grewe (Universität Tübingen) for technical assistance in fermentations, and Dr. P. Schmieder (FMP, Berlin-Buch) for measurement of 15N NMR spectra.
Thermochemical and Physical Properties of Element 112FNR HREF="nss"> FN ID="nss"> We are indebted to the staff of the U-400 cyclotron for providing intense beams of 48Ca. This work was supported in part by the Russian Foundation for Basic Research (Grant 07-03-00430) and by the Swiss National Science Foundation (Grant 200020-109171).
Cationic RuII Complexes with N-Heterocyclic Carbene Ligands for UV-Induced Ring-Opening Metathesis PolymerizationFNR HREF="nss"> FN ID="nss"> This work was supported by the Deutsche Forschungsgemeinschaft (DFG, project BU 2174-2-1), by the Federal Government of Germany and the Freistaat Sachsen.
Sensitized Detection of Inhibitory Fragments and Iterative Development of Non-Peptidic Protease Inhibitors by Dynamic Ligation ScreeningFNR HREF="nss"> FN ID="nss"> We wish to thank Samuel Beligny, Angelika Ehrlich, Franziska Hinterleitner, Dagmar Krause, Jörn Saupe, Bernhard Schmikale, and Walter Verheyen for technical support. We also acknowledge Jeroen R. Mesters and Koen H. Verschueren for discussions. Work at the FMP was supported by the DFG (Ra 895-2-5), by the government of Catalunya (stipend to A.I.L.), and by Boehringer Ingelheim Pharma. Work at Lübeck University was supported by the DFG (Hi 611-4-1), the Schleswig-Holstein Innovation Fund, the Sino-German Center for the Promotion of Research, Bejing (GZ 233-202-6), and the European Commission through its SEPSDA project (SP22-CT-2004-003831). J.R. and R.H. thank the Fonds der Chemischen Industrie for continuous support.
Visual Observation of Redistribution and Dissolution of Palladium during the Suzuki-Miyaura ReactionFNR HREF="nss"> FN ID="nss"> The Natural Sciences and Engineering Research Council of Canada is acknowledged for support of this research in terms of operating grants to C.M.C., H.P.L., and J.H.H., and for scholarships to K.M. Queen's University is acknowledged for support to K.M.