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Table of contents
8133
Cover Picture: An Unlockable–Relockable Iron Cage by Subcomponent Self‐Assembly (Angew. Chem. Int. Ed. 43/2008)
Inside Cover: Si@Al56[N(2,6‐iPr2C6H3)SiMe3]12: The Largest Neutral Metalloid Aluminum Cluster, a Molecular Model for a Silicon‐Poor Aluminum–Silicon Alloy? (Angew. Chem. Int. Ed. 43/2008)
Huber, Michael
/ Schnepf, Andreas
/ Anson, Christopher E.et al.
| 2008
Sensing on a Molecular Level-Chemistry at the Interface of Information Technology Generous financial support by the MPI für Kohlenforschung and the DFG (Emmy Noether program TR 542-3), the Fond der Chemischen Industrie (FCI), the Merck Research Laboratories (Rahway, NJ), and the Nordrhein-Westfälische Akademie der Wissenschaften is gratefully acknowledged.
Navigating the Folding Energy Landscape of Green Fluorescent Protein We thank Dr. Hendrik Dietz for scientific inspiration and exploratory work. Financial support from DFG (grant RI 990-3-1) is gratefully acknowledged.
Carbon Pyramidalization in Fullerene Cages Induced by the Endohedral Cluster: Non-Scandium Mixed Metal Nitride Clusterfullerenes We cordially thank K. Leger, S. Schiemenz, and F. Ziegs for their technical assistance. S.Y. thanks the University of Science and Technology of China (USTC) for Startup funding (No.: ZC9850290028). Financial support for A.P. from DAAD and AvH is gratefully acknowledged.
Si@Al56[N(2,6-iPr2C6H3)SiMe3]12: The Largest Neutral Metalloid Aluminum Cluster, a Molecular Model for a Silicon-Poor Aluminum-Silicon Alloy? We thank the Deutsche Forschungsgemeinschaft (DFG), the DFG Research Center of Functional Nanostructures (CFN), the Karlsruhe Institute of Technology (KIT), and the Fonds der Chemischen Industrie for financial support. We also thank Dr. G. Fischer and Prof. Dr. F. Breher for SQUID and EPR measurements.
Accurate Melting Temperatures for Neon and Argon from Ab Initio Monte Carlo Simulations We thank K. Szalewicz for providing the routines for the SAPT three-body potential and A. Hermann for technical support. This work was supported by the Royal Society of New Zealand (Marsden grant 07-MAU-016), the Swedish Research Council (VR), and the Durmont d'Urville PHC programme (15883VC) of the French and New Zealand governments.
Copper-Catalyzed Asymmetric Conjugate Addition of Aryl Aluminum Reagents to Trisubstituted Enones: Construction of Aryl-Substituted Quaternary Centers We thank the European Community (Marie Curie Early Stage Researcher Training, MEST-CT-2005-019780) for financial support.
Semisynthesis of a Glycosylphosphatidylinositol-Anchored Prion Protein Financial support from the Max Planck Society, the Deutsche Forschungsgemeinschaft, the Fonds der chemischen Industrie, the Swiss National Science Foundation (SNF grant 205321-107651), and ETH Zürich is gratefully acknowledged. The authors thank J. Tatzelt and M. Engelhard for helpful discussions.
A Genetically Encoded Boronate-Containing Amino Acid We thank Dr. Vaughn Smider, Chang Liu, Jeremy Mills, and Emily Remba for assistance and helpful discussion. This work is supported by NIH grant R01 GM062159, US Department of Energy, Division of Materials Sciences, under Award No. DE-FG03-00ER46051, and the Skaggs Institute for Chemical Biology.
A Palladium-Catalyzed Dehydrogenative Diamination of Terminal Olefins We are grateful for generous financial support from the National Institute of General Medical Sciences, National Institutes of Health (grant no. GM083944-01) and the Camille and Henry Dreyfus Foundation.
Incorporating Phosphaalkenes into Oligoacetylenes This work was supported by the Swedish Research Council, the Göran Gustafssons Foundation, and the Carl Trygger Foundation.
An Immobilization Method of Chiral Quaternary Ammonium Salts onto Polymer Supports This work was financially supported by a Grant-in-Aid from the Ministry of Education, Culture, Sports, Science, and Technology (Japan).
Towards the Ultimate Size Limit of the Memory Effect in Spin-Crossover Solids The authors thank Mme Corine Reibel (LPMC, Montpellier, France) for magnetic measurements. Financial supports from the CNRS, the Université Montpellier II, the ANR NANOMOL project and the European Network of Excellence MAGMANET are acknowledged.
Two-Component Liquid Crystals as Chiral Reaction Media: Highly Enantioselective Photodimerization of an Anthracene Derivative Driven by the Ordered Microenvironment We acknowledge Dr. Toshimi Shimizu and Dr. Hiroyuki Minamikawa (AIST), and Prof. Junji Watanabe and Dr. Masatoshi Tokita (TIT) for XRD measurements. We would like to thank Prof. Takashi Kato (UT) for use of the DSC equipment. A part of this work was financially supported by a Grants-in-Aid for Exploratory Research (No. 16655043) from MEXT (Japan).
Two‐Component Liquid Crystals as Chiral Reaction Media: Highly Enantioselective Photodimerization of an Anthracene Derivative Driven by the Ordered Microenvironment
A General and Selective Copper-Catalyzed Cross-Coupling of Tertiary Grignard Reagents with Azacyclic Electrophiles This work was supported by the DFG (Emmy Noether Programme). We thank Prof. Carsten Bolm for continued support.
Distinctly Different Reactivities of Two Similar Polyoxoniobates with Hydrogen Peroxide The research was supported by the U.S. Department of Energy, Office of Basic Energy Science (grant number DE-FG02-05ER15693) and the National Science Foundation (grant EAR0814242). We are also grateful to Dr. May Nyman and Dr. Travis M. Anderson (Sandia National Laboratories) for generous advice and a gift of hydrous niobium oxide.
An Efficient Approach to Substituted 1,5,7,8,9‐Pentahydrocyclopenta[h]‐2‐Benzopyran‐3‐one Derivatives by a Palladium‐Catalyzed Tandem Reaction of 2,7‐Alkadiynylic Carbonates with 2,3‐Allenoic Acids
An Efficient Approach to Substituted 1,5,7,8,9-Pentahydrocyclopenta[h]-2-Benzopyran-3-one Derivatives by a Palladium-Catalyzed Tandem Reaction of 2,7-Alkadiynylic Carbonates with 2,3-Allenoic Acids Financial support from the State Key Basic Research & Development Program (2006CB806105) and the National Natural Science Foundation of China (20732005) are greatly appreciated. We also thank J. Chen for reproducing the results presented in Table 2, entries 2 and 8, and Scheme 2.
Stepwise Cosensitization of Nanocrystalline TiO2 Films Utilizing Al2O3 Layers in Dye-Sensitized Solar Cells This work was supported by the Korea Science and Engineering Foundation (KOSEF) through the National Research Lab. Program funded by the Ministry of Science and Technology (No. R0A-2005-000-10034-0), and BK-21 (2006). M.G. and M.K.N. thank Swiss Federal Office for Energy (OFEN). E.P. thanks the Spanish MEC for the CONSOLIDER-HOPE 0007-2007, and the CTQ2007-60746-BQU project.
Functionalization of Imprinted Nanopores in Nanometer-Thin Organic Materials This work was supported by a US National Science Foundation CAREER Award (CHE-0349315), National Institutes of Health grant (1R01HL079147-01) and a FedEx Institute of Technology Innovation Award. We thank Lou Boykins from the Integrated Microscopy Center at the University of Memphis for help with electron microscopy.
Colossal Pressure-Induced Lattice Expansion of Graphite Oxide in the Presence of Water High-pressure experiments at HASYLAB were supported by the GFZ Potsdam under the MAX80 program. This work was partially supported by the Agence Nationale de la Recherche grant NT05-3_42601. Some of the high-pressure experiments (A.T.) were performed at the Bayerisches Geoinstitut under the EU "Research Infrastructures: Transnational Access" Programme (Contract No. 505320 (RITA)-High Pressure). We thank Prof. L. Dubrovinsky for providing access to facilities at BGI and discussions.
Photoelectrochemistry with Ordered CdS Nanoparticle-Relay or Photosensitizer-Relay Dyads on DNA Scaffolds This research was supported by the NanoSci-ERA (Nano Licht Project).
High Internal Phase Emulsions Stabilized Solely by Functionalized Silica Particles This work was supported by the Challenging Engineering Programme (EP-E007538-1) of the UK Engineering and Physical Science Council (EPSRC) and Halliburton Energy Services. An ORS Award for V.O.I. is greatly acknowledged.
Shape Development and Structure of a Complex (Otoconia-Like?) Calcite-Gelatine Composite We gratefully acknowledge the Fonds der Chemischen Industrie for generous support. We are also grateful to Dr. G. Auffermann and A. Völzke for elemental analyses, H. Dallmann (TU Dresden) for thermal analyses, and Dr. U. Burkhardt for density measurements. We thank Prof. H. Lichte (TU Dresden) for the possibility to perform TEM measurements at the Triebenberg Laboratory and Dr. S. Wirth for fruitful discussions. Finally, we thank Prof. T. Zahnert and Dr. Y. Yarin (Universitätsklinikum der TU Dresden) for the SEM images of biogenic otoconia; coloring of the images was performed by Dipl.-Ing. H. Tlatlik (MPI CPfS).
Ruthenium-Catalyzed Cycloaddition of Nitrile Oxides and Alkynes: Practical Synthesis of Isoxazoles Financial support from the Skaggs Institute for Chemical Biology and Pfizer, Inc. is gratefully acknowledged. We thank Prof. K. B. Sharpless for stimulating discussions and advice.
Dipositively Charged Protonated a3 and a2 Ions: Generation by Fragmentation of [La(GGG)(CH3CN)2]3+ This study was supported by the Natural Sciences and Engineering Research Council (NSERC) of Canada and made possible by the facilities of the Shared Hierarchical Academic Research Computing Network (SHARCNET: www.sharcnet.ca). We thank Dr. Julia Laskin for helpful discussions on the RRKM modeling.
Polytriphenylene Dendrimers: A Unique Design for Blue-Light-Emitting Materials This work was financially supported by the Deutsche Forschungsgemeinschaft (DFG) within the frame of the Sonderforschungsbereich (SFB)625. G. Z. gratefully acknowledges the Alexander von Humboldt Stiftung for a research fellowship.
An Unlockable-Relockable Iron Cage by Subcomponent Self-Assembly This work was supported by the Walters-Kundert Charitable Trust, the Royal Society, the Swiss National Science Foundation, and the Academy of Finland (122350), the Graduate School of Organic Chemistry and Chemical Biology (K.B.) and the Marie Curie IIF Scheme of the 7th EU Framework Program (P.M.).
Carbenes Stabilized by Ylides: Pushing the Limits Generous financial support from the MPG, the Spanish Ministerio de Educación y Ciencia (fellowship for M.A.), and the Fonds der Chemischen Industrie is gratefully acknowledged.
Synthesis of an Energetic Nitrate Ester This work was supported at the Los Alamos National Laboratory by the Joint DOE-DoD Munitions Technology Development Program and at the Naval Research Laboratory by the office of Naval Research, Mechanics Division.
Triarylphosphanes with Dendritically Arranged Tetraethylene Glycol Moieties at the Periphery: An Efficient Ligand for the Palladium-Catalyzed Suzuki-Miyaura Coupling Reaction This work was supported by a Grant-in-Aid for Scientific Research on Priority Areas ("Synergy of Elements" and "Chemistry of Concerto Catalysis") from the Ministry of Education, Culture, Sports, Science, and Technology (Japan).
Triarylphosphanes with Dendritically Arranged Tetraethylene Glycol Moieties at the Periphery: An Efficient Ligand for the Palladium‐Catalyzed Suzuki–Miyaura Coupling Reaction